Spatial distribution of 241Am, 137Cs, 238Pu, 239,240Pu and 241Pu over 17 year periods in the Ravenglass saltmarsh, Cumbria, UK

Ninety five surface scrape samples were collected at the Ravenglass saltmarsh and analysed for radionuclides by alpha spectrometry (Pu-238 and Pu-239,Pu-240), gamma spectrometry (Am-241 and Cs-137) and liquid scintillation counting ((241) Pu). Both Am-241 and Cs-137 activities are compared with those reported by Horrill [1983. Concentrations and spatial distribution of radioactivity in an ungrazed saltmarsh. In: Coughtrey, P.J. (Ed.), Ecological Aspects of Radionuclide Release. British Ecological Society Special Publication No. 3. Blackwell, Oxford. pp. 119-215.] Significant decreases in activities for both radionuclides were observed which is caused by the declining levels of discharges from the Sellafield nuclear reprocessing plant since the 1980s. It has been concluded that the spatial distribution of these radionuclides are controlled by the tidal currents and the clay contents in the sediments. There is evidence of surface erosion of the saltmarsh and redistribution of radionuclides in the saltmarsh using isotopic ratios of measured Pu. (C) 2009 Elsevier Ltd. All rights reserved.