A high-efficiency reactor for the pulsed plasma conversion of methane

被引:62
|
作者
Yao, SL [1 ]
Suzuki, E [1 ]
Meng, N [1 ]
Nakayama, A [1 ]
机构
[1] Res Inst Innovat Technol Earth, Catalysis Sci Lab, Kyoto 6190292, Japan
关键词
pulsed plasma; methane; acetylene; point-to-point reactor; energy efficiency;
D O I
10.1023/A:1014843425384
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The authors recently developed a high-frequency pulsed plasma process for Methane conversion to acetylene and hydrogen using a co-axial cylindrical (CAC) type of reactor. The energy, efficiency, represented by methane conversion rate per unit input energy has been improved so that such a pulsed plasma has potential for commercial acetylene production. A pulsed plasma consists of a pulsed corona discharge and a pulsed spark discharge, Most of energy, is injected over the duration of the pulsed spark discharge, Methane conversion using this kind of pulsed plasma is a kind of pyrolysis enhanced by, the pulsed spark discharge. In this study, a point-to-point (PTP) type of reactor that can produce a discharge channel over the duration of a pulse discharge was used for the pulsed plasma conversion of methane. The energy efficiency and carbon formation on electrodes have been improved. The influences of pulse frequency, and pulse voltage on methane conversion rate and product selectivity it-ere investigated The features of methane conversion using PTP and CA C reactors were discussed.
引用
收藏
页码:225 / 237
页数:13
相关论文
共 50 条
  • [1] A High-Efficiency Reactor for the Pulsed Plasma Conversion of Methane
    S.L. Yao
    E. Suzuki
    N. Meng
    A. Nakayama
    Plasma Chemistry and Plasma Processing, 2002, 22 : 225 - 237
  • [2] Analysis of a high frequency pulsed plasma for methane conversion.
    Yao, SL
    Suzuki, E
    Nakayama, A
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2000, 220 : U389 - U389
  • [3] Deciphering high-efficiency solar-thermochemical energy conversion process of heat pipe reactor for steam methane reforming
    Ma, Jing
    Jiang, Bo
    Si-ma, Wang
    Yu, Kewei
    Lv, Zheng
    Gao, Yuming
    Yuan, Dazhong
    Tang, Dawei
    FUEL, 2022, 326
  • [4] A compact and high-efficiency electrified reactor for hydrogen production by methane steam reforming
    Ma, Jing
    Jiang, Bo
    Gao, Yuming
    Yu, Kewei
    Lv, Zheng
    Si-ma, Wang
    Yuan, Dazhong
    Tang, Dawei
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (98) : 41421 - 41431
  • [5] NiO/ZnO heterojunction nanorod catalyst for high-efficiency electrochemical conversion of methane
    Kim, Cheolho
    Min, Heewon
    Kim, Junmin
    Sul, Jiwon
    Yang, Jiwoo
    Moon, Jun Hyuk
    APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY, 2023, 323
  • [6] Stable kilohertz spark discharges for high-efficiency conversion of methane to hydrogen and acetylene
    Li, Xiao-Song
    Lin, Can-Kun
    Shi, Chuan
    Xu, Yong
    Wang, You-Nian
    Zhu, Ai-Min
    JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2008, 41 (17)
  • [7] Methane conversion by repetitive nanosecond pulsed plasma
    Lotfalipour, R.
    Ghorbanzadeh, A. M.
    Mahdian, A.
    JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2014, 47 (36)
  • [8] Conversion of Methane in Plasma of Pulsed Nanosecond Discharges
    Kuznetsov, Dmitrii L.
    Uvarin, Viktor V.
    Filatov, Igor E.
    IEEE TRANSACTIONS ON PLASMA SCIENCE, 2021, 49 (09) : 2604 - 2612
  • [9] Methane conversion using a high-frequency pulsed plasma: Discharge features
    Yao, SL
    Nakayama, A
    Suzuki, E
    AICHE JOURNAL, 2001, 47 (02) : 419 - 426
  • [10] Methane conversion using a high-frequency pulsed plasma: Important factors
    Yao, SL
    Nakayama, A
    Suzuki, E
    AICHE JOURNAL, 2001, 47 (02) : 413 - 418