Gel-emulsion templated polymeric monoliths for efficient removal of particulate matters

被引:29
|
作者
Liu, Jianfei [1 ]
Li, Min [2 ]
Wang, Pei [2 ]
Liu, Kaiqiang [2 ]
Fang, Yu [2 ]
机构
[1] Shaanxi Normal Univ, Sch Mat Sci & Engn, Key Lab Appl Surface & Colloid Chem, Minist Educ, Xian 710062, Shaanxi, Peoples R China
[2] Shaanxi Normal Univ, Sch Chem & Chem Engn, Key Lab Appl Surface & Colloid Chem, Minist Educ, Xian 710062, Shaanxi, Peoples R China
关键词
Gel-emulsions; Porous polymeric monoliths; Acidified cotton; Particulate matter; Air pollution; PHASE PICKERING EMULSIONS; AIR-POLLUTION; COMPOSITE MEMBRANE; GAS; COLUMNS; HIPES; PM2.5;
D O I
10.1016/j.cej.2018.01.110
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this work, a series of porous polymeric monoliths with densities as low as similar to 0.060 g/cm(3) were prepared by employing some newly created gel-emulsions as templates, of which acidified cotton was utilized for the first time as an efficient stabilizer. The monoliths as obtained could be purified by simple washing and dried at ambient conditions. Moreover, they showed strong affinity to particulate matters (PMs). Adsorption tests revealed that the saturated adsorption capacity of one of the monoliths (M8) to PM2.5 could reach similar to 520 mg/g and the removal efficiency exceeds 93% at ambient conditions, a prominent result considering the collective advantages of the monolith. Importantly, the monoliths after adsorption can be recovered and re-used via simple washing and drying. More importantly, the stabilizer as created is so efficient that 0.1% (w/v, cotton to the volume of the continuous phase) is enough to stabilize the gel emulsions. Considering the excellence in performance, low cost in preparation, and convenience in regeneration, we believe that the monoliths are strong candidates for real-life applications.
引用
收藏
页码:14 / 21
页数:8
相关论文
共 19 条
  • [1] Gel-emulsion templated polymeric aerogels for solar-driven interfacial evaporation and electricity generation
    Liu, Jianfei
    Chen, Xiangli
    Yang, Hui
    Tang, Jiaqi
    Miao, Rong
    Liu, Kaiqiang
    Fang, Yu
    [J]. MATERIALS CHEMISTRY FRONTIERS, 2021, 5 (04) : 1953 - 1961
  • [2] Gel-Emulsion-Templated Polymeric Aerogels for Water Treatment by Organic Liquid Removal and Solar Vapor Generation
    Liu, Jianfei
    Yang, Hui
    Liu, Kaiqiang
    Miao, Rong
    Fang, Yu
    [J]. CHEMSUSCHEM, 2020, 13 (04) : 749 - 755
  • [3] Emulsion-Templated Porous Polymers for Efficient Dye Removal
    Uzum, Gulenay
    Ozmen, Busra Akin
    Akgul, Ebru Tekneci
    Yavuz, Erdem
    [J]. ACS OMEGA, 2022, 7 (18): : 16127 - 16140
  • [4] Compressible porous hybrid monoliths: preparation via a low molecular mass gelators-based gel-emulsion approach and exceptional performances
    Chen, Xiangli
    Liu, Lingling
    Liu, Kaiqiang
    Miao, Qing
    Lu, Yanchao
    Fang, Yu
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (48) : 24322 - 24332
  • [5] One-step preparation of emulsion-templated amino-functionalized porous organosilica monoliths for highly efficient Cr(VI) removal
    Zhang, Hongxia
    Lu, Jieli
    Peng, Junxia
    Du, Guanqun
    Peng, Haonan
    Fang, Yu
    [J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2018, 555 : 8 - 17
  • [6] Polyelectrolyte aerogels with regeneration capacity for efficient removal of particulate matters
    Wu, Wenna
    Ma, Lin
    Chen, Xiaoli
    Liu, Li
    Dong, Shuli
    Zou, Huiling
    Hao, Jingcheng
    [J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2022, 625 : 446 - 456
  • [7] Configuration of an efficient seawater pretreatment system for simultaneous organic and particulate matters removal
    Hyun, Kil-Soo
    [J]. DESALINATION AND WATER TREATMENT, 2011, 33 (1-3) : 295 - 299
  • [8] Compressible porous hybrid monoliths: preparation via a low molecular mass gelators-based gel-emulsion approach and exceptional performances (vol 3, pg 24322, 2015)
    Chen, Xiangli
    Liu, Lingling
    Liu, Kaiqiang
    Miao, Qing
    Lu, Yanchao
    Fang, Yu
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2016, 4 (02) : 684 - 684
  • [9] Nanofibrous, hierarchically porous poly(ether sulfone) xerogels templated from gel emulsions for removing organic vapors and particulate matters
    Xie, Jingang
    Liu, Chao
    Gui, Haoguan
    Ding, Yunsheng
    Yao, Chao
    Zhang, Tao
    [J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2022, 648
  • [10] High performance microwave absorption of light weight and porous non-carbon-based polymeric monoliths via a gel emulsion template
    Zhang, Cheng
    He, Yuting
    Song, Qingwen
    Tan, Yanjun
    Ren, Yubo
    Cheng, Wei
    Miao, Runfeng
    Fan, Wei
    Zhou, Deyun
    [J]. POLYMER CHEMISTRY, 2022, 13 (12) : 1672 - 1684