High hydrogen production from glycerol or glucose by electrohydrogenesis using microbial electrolysis cells

被引:184
|
作者
Selembo, Priscilla A. [2 ]
Perez, Joe M. [2 ]
Lloyd, Wallis A. [2 ]
Logan, Bruce E. [1 ]
机构
[1] Penn State Univ, Dept Civil & Environm Engn, University Pk, PA 16802 USA
[2] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA
关键词
MEC; Electrohydrogenesis; Biocatalyzed electrolysis; Hydrogen; Glycerol; Glucose; Biodiesel; FUEL-CELLS; CRUDE GLYCEROL; PSEUDOMONAS-AERUGINOSA; ELECTRICITY-GENERATION; BIOHYDROGEN PRODUCTION; BIODIESEL PRODUCTION; COMMUNITY ANALYSIS; MIXED CULTURES; FERMENTATION; PROPIONATE;
D O I
10.1016/j.ijhydene.2009.05.002
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The use of glycerol for hydrogen gas production was examined via electrohydrogenesis using microbial electrolysis cells (MECs). A hydrogen yield of 3.9 mol-H-2/mol was obtained using glycerol, which is higher than that possible by fermentation, at relatively high rates of 2.0 +/- 0.4 m(3)/m(3) d (E-ap = 0.9 V). Under the same conditions, hydrogen was produced from glucose at a yield of 7.2 mol-H-2/mol and a rate of 1.9 +/- 0.3 m(3)/m(3) d. Glycerol was completely removed within 6 h, with 56% of the electrons in intermediates (primarily 1,3-propanediol), with the balance converted to current, intracellular storage products or biomass. Glucose was removed within 5 h, but intermediates (mainly propionate) accounted for only 19% of the electrons. Hydrogen was also produced using the glycerol byproduct of biodiesel fuel production at a rate of 0.41 +/- 0.1 m(3)/m(3) d. These results demonstrate that electrohydrogenesis is an effective method for producing hydrogen from either pure glycerol or glycerol byproducts of biodiesel fuel production. (C) 2009 International Association for Hydrogen Energy. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:5373 / 5381
页数:9
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