Migration of plutonium in a simulated engineered barrier system consisting of waste glass and compacted bentonite

被引:2
|
作者
Inagaki, Y [1 ]
Saito, R [1 ]
Furuya, H [1 ]
Idemitsu, K [1 ]
Arima, T [1 ]
Banbu, T [1 ]
Maeda, T [1 ]
Matsumoto, S [1 ]
Tamura, Y [1 ]
Kikkawa, S [1 ]
机构
[1] Kyushu Univ, Dept Nucl Engn, Fukuoka 8128581, Japan
关键词
D O I
10.1557/PROC-556-1083
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In a simulated engineered barrier system consisting of a simulated HLW glass doped with Pu, a compacted bentonite and water under reducing conditions, migration tests of Pu from the glass into the bentonite through water were performed. The following results were obtained: (1) The presence of bentonite enhances the glass dissolution while it has no remarkable influence on the concentration of Pu dissolved species in the solution. (2) Only a small part of the leached Pu, which may correspond to the dissolved species, can diffuse into the bentonite with the apparent diffusion coefficient of 3 x 10(-14)m(2)/s. (3) Interactions between the glass and the bentonite have no remarkable influence on the diffusion of Pu.
引用
收藏
页码:1083 / 1090
页数:4
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