Facile synthesis of mesoporous detonation nanodiamond-modified layers of graphitic carbon nitride as photocatalysts for the hydrogen evolution reaction

被引：27
|
作者：
Haleem, Yasir A. [1 ]
He, Qun [1 ]
Liu, Daobin [1 ]
Wang, Changda [1 ]
Xu, Weiyu [1 ]
Gan, Wei [1 ]
Zhou, Yu [1 ]
Wu, Chuangqiang [1 ]
Ding, Yanwei [2 ]
Song, Li [1 ]
机构：
[1] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, CAS Ctr Excellence Nanosci, Hefei 230029, Anhui, Peoples R China
[2] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Hefei, Peoples R China
来源：
RSC ADVANCES | 2017年 / 7卷 / 25期
基金：
中国国家自然科学基金;
关键词：
VISIBLE-LIGHT; SURFACE FUNCTIONALIZATION; BAND-STRUCTURE; NANOCOMPOSITES; DIAMOND; G-C3N4; WATER; ELECTRODES; NANOSCALE;
D O I：
10.1039/c7ra02178j
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The hydrogen evolution reaction (HER) may contribute substantially to energy resources in the future through solar energy conversion. In this study, mesoporous graphitic carbon nitride (g-C3N4) layers modified by detonation nanodiamond (DND) were synthesized by condensation from urea to obtain a robust and efficient hybrid (g-C3N4-DND) photocatalyst for the HER. Our characterizations revealed that no significant structural changes occurred in g-C3N4 during the synthesis of the g-C3N4-DND hybrid. Compared with pure g-C3N4, hydrogen production increased by almost 50% when using the hybrid photocatalyst due to the synergetic effect of the enhanced charge transfer, high surface area and low recombination rate of the photogenerated charge carriers.
引用
收藏
页码：15390 / 15396
页数：7
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