A non-noble Cr-Ni-based catalyst for the oxygen reduction reaction in alkaline polymer electrolyte fuel cells

被引:9
|
作者
Faubert, P. [1 ]
Kondov, I. [2 ]
Qazzazie, D. [3 ]
Yurchenko, O. [4 ]
Mueller, C. [1 ]
机构
[1] Univ Freiburg, Dept Microsyst Engn IMTEK, Lab Proc Technol, D-79110 Freiburg, Germany
[2] Karlsruhe Inst Technol, Steinbuch Ctr Comp, Hermann von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany
[3] Univ Freiburg, Dept Microsyst Engn IMTEK, Lab Sensors, D-79110 Freiburg, Germany
[4] Univ Freiburg, Freiburg Mat Res Ctr FMF, D-79104 Freiburg, Germany
关键词
ANION-EXCHANGE MEMBRANES; NAFION MEMBRANES; DYNAMICS; TRANSITION; VEHICLES;
D O I
10.1557/mrc.2018.13
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report on a new type of polymer electrolyte fuel cell based on a hydroxide ion conductive polymer combined with a non-noble chromium-nickel (Cr-Ni) catalyst for the oxygen reduction reaction (ORR). We study variable fractions of Cr in Ni by density functional theory simulating the thermodynamic potentials characterizing the ORR. We found increased ORR catalytic activity employing the rotating disk electrode technique. The polarization curve and power densities measured for the constructed fuel cell indicate considerable performance improvement with the Cr-Ni catalyst. Thus we expect that this kind of fuel cell may open up alternative routes in fuel cell research using non-noble catalysts.
引用
收藏
页码:160 / 167
页数:8
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