Onsager Reciprocity in Premelting Solids

被引：11

作者：

Peppin, S. S. L. ^{[1
]}

Spannuth, M. J. ^{[1
]}

Wettlaufer, J. S. ^{[1
,2
,3
]}

机构：

[1] Yale Univ, Dept Geol & Geophys, New Haven, CT 06520 USA

[2] Yale Univ, Dept Phys, New Haven, CT 06520 USA

[3] Nord Inst Theoret Phys, S-10691 Stockholm, Sweden

来源：

JOURNAL OF STATISTICAL PHYSICS | 2009年 / 134卷 / 04期

基金：

美国国家科学基金会;

关键词：

Reciprocity; Premelting; Diffusion; Soret effect; Dufour effect; Surface phase transitions; Colloids; TRANSPORT PROCESSES; DYNAMICS; ICE; SYSTEMS; FORCES; GLASS; HEAT;

D O I：

10.1007/s10955-009-9699-z

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

The diffusive motion of foreign particles dispersed in a premelting solid is analyzed within the framework of irreversible thermodynamics. We determine the mass diffusion coefficient, thermal diffusion coefficient and Soret coefficient of the particles in the dilute limit, and find good agreement with experimental data. In contrast to liquid suspensions, the unique nature of premelting solids allows us to derive an expression for the Dufour coefficient and independently verify the Onsager reciprocal relation coupling diffusion to the flow of heat.

引用

页码：701 / 708

页数：8

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