Source apportionment of polycyclic aromatic hydrocarbons in the terrestrial soils of King George Island, Antarctica

被引:19
|
作者
Deelaman, Woranuch [1 ]
Pongpiachan, Siwatt [2 ]
Tipmanee, Danai [3 ]
Suttinun, Oramas [1 ]
Choochuay, Chomsri [1 ]
Iadtem, Natthapong [1 ]
Charoenkalunyuta, Teetat [4 ]
Promdee, Kittiphop [5 ]
机构
[1] Prince Songkla Univ Hat Yai Campus, Fac Environm Management, Songkhla 90112, Thailand
[2] Natl Inst Dev Adm NIDA, NIDA Ctr Res & Dev Disaster Prevent & Management, Sch Social & Environm Dev, 118 Moo 3,Sereethai Rd, Bangkok 10240, Thailand
[3] Prince Songkla Univ, Fac Technol & Environm, Phuket Campus 80 M-1 Kathu, Phuket 83120, Thailand
[4] Chulalongkorn Univ, Dept Survey Engn, Bangkok 10330, Thailand
[5] Chulachomklao Royal Mil Acad, Dept Environm Sci, Nakhon 26001, Thailand
关键词
Polycyclic aromatic hydrocarbon; PAH; Terrestrial soil; King George island; Binary diagnostic ratio; Source apportionment; Principal components analysis; Hierarchical cluster analysis; ECOLOGICAL RISK-ASSESSMENT; FINE ORGANIC AEROSOL; SOURCE IDENTIFICATION; MOLECULAR MARKERS; SURFACE SEDIMENTS; MARINE-SEDIMENTS; RIVER-BASIN; PAH SOURCE; PCBS; ENVIRONMENT;
D O I
10.1016/j.jsames.2020.102832
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
This study employed chemical characterisation to determine the source of polycyclic aromatic hydrocarbons (PAHs) in the terrestrial soils of King George Island, Antarctica. The total concentrations of 12 PAHs in the samples of terrestrial soils collected at 44 sites ranged from 1.83 to 32.9 ng g(-1) with an average value of 10.8 +/- 8.22 ng g(-1). The concentrations of these PAHs were relatively lower compared with those found in other studies in other locations. The spatial distributions of PAHs showed the highest concentrations to be in areas adjacent to the Great Wall Station and the road network, and light molecular weight PAHs were predominant. Threeand four-ring PAHs were the most abundant, representing 48.3% and 27.1% of the total, respectively. Although the binary diagnostic ratios indicated petrogenic sources as the main PAH-emission sources, principal components analysis and hierarchical cluster analysis suggested that electricity generators (22.84%) and light-duty gasoline (18.94%) are the main sources in the soil of King George Island, Antarctica.
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页数:13
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