Local and long-range transport influences on PM2.5 at a cities-cluster in northern China, during summer 2008

被引:15
|
作者
Gao, Lijie [1 ]
Tian, Yingze [1 ]
Zhang, Caiyan [1 ]
Shi, Guoliang [1 ]
Hao, Huize [1 ]
Zeng, Fang [1 ]
Shi, Chunli [1 ]
Zhang, Meigen [2 ]
Feng, Yinchang [1 ]
Li, Xiang [1 ,3 ]
机构
[1] Nankai Univ, Coll Environm Sci & Engn, State Environm Protect Key Lab Urban Ambient Air, Tianjin 300071, Peoples R China
[2] Chinese Acad Sci, Inst Atmospher Phys, Beijing 100029, Peoples R China
[3] Univ Georgia, Dept Comp Sci, Athens, GA 30602 USA
来源
PARTICUOLOGY | 2014年 / 13卷
基金
中国国家自然科学基金;
关键词
Local influence; Regional influence; Joint potential source contribution function; Hierarchical cluster analysis; POSITIVE MATRIX FACTORIZATION; SOURCE APPORTIONMENT; CHEMICAL-COMPOSITION; PARTICULATE MATTER; SOURCE LOCATIONS; DUST SOURCES; AEROSOL; POLLUTION; PM10; CITY;
D O I
10.1016/j.partic.2013.06.006
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Hourly PM2.5 concentrations were observed simultaneously at a cities-cluster comprising 10 cities/towns in Hebei province in China from July 1 to 31, 2008. Among the 10 cities/towns, Baoding showed the highest average concentration level (161.57 mu g/m(3)) and Yanjiao exhibited the lowest (99.35 mu g/m(3)). These observed data were also studied using the joint potential source contribution function with 24-h and 72-h backward trajectories, to identify more clearly the local and countrywide-scale long-range transport sources. For the local sources, three important influential areas were found, whereas five important influential areas were defined for long-range transport sources. Spatial characteristics of PM2.5 were determined by multivariate statistical analyses. Soil dust, coal combustion, and vehicle emissions might be the potential contributors in these areas. The results of a hierarchical cluster analysis for back trajectory endpoints and PM2.5 concentrations datasets show that the spatial characteristics of PM2.5 in the cities-cluster were influenced not only by local sources, but also by long-range transport sources. Different cities in the cities-cluster obtained different weighted contributions from local or long-range transport sources. Cangzhou, Shijiazhuang, and Baoding are near the source areas in the south of Hebei province, whereas Zhuozhou, Yangfang, Yanjiao, Xianghe, and Langfang are close to the sources areas near Beijing and Tianjin. (C) 2013 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:66 / 72
页数:7
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