Time-dependent renormalized Redfield theory

被引：8
|
作者：
Kimura, Akihiro [1 ]
机构：
[1] Nagoya Univ, Grad Sch Sci, Dept Phys, Chikusa Ku, Furo Cho, Nagoya, Aichi 4648602, Japan
来源：
CHEMICAL PHYSICS LETTERS | 2016年 / 645卷
关键词：
ELECTRON-TRANSFER; PHOTOSYSTEM-II; ENERGY; FORSTER; PHOTOSYNTHESIS; COHERENCE; COMPLEXES; EQUATIONS; DYNAMICS; STATES;
D O I：
10.1016/j.cplett.2015.12.047
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In this Letter, we apply time-dependent renormalization to the perturbation term in modified Redfield theory. We show the general reaction rate formula, which is numerically calculable, and discuss new findings about quantum vibrational effects with respect to the modified Redfield formalism. Using the renormalization treatment, we discuss the analytical origins of its increasing reaction rate with the present, more accurate formalism. (C) 2015 Elsevier B.V. All rights reserved.
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页码：123 / 126
页数：4
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