Room temperature exciton-polaritons in high-quality 2D Ruddlesden-Popper perovskites (BA)2(MA)n-1PbnI3n<bold>+</bold>1 (n <bold>=</bold> 3, 4)

被引:7
|
作者
Ouyang, Chenxing [1 ]
Li, Yao [2 ]
Fu, Xianwei [3 ]
Zeng, Zhouxiaosong [1 ]
Huang, Lanyu [1 ]
Liu, Siman [1 ]
Wang, Xiao [1 ]
Gao, Tingge [2 ]
Pan, Anlian [3 ]
机构
[1] Hunan Univ, Sch Phys & Elect, Key Lab Micronano Phys & Technol Hunan Prov, Changsha 410082, Hunan, Peoples R China
[2] Tianjin Univ, Inst Mol Plus, Tianjin Key Lab Mol Optoelect Sci, Tianjin 300072, Peoples R China
[3] Hunan Univ, Coll Mat Sci & Engn, Changsha 410082, Hunan, Peoples R China
基金
中国国家自然科学基金;
关键词
D O I
10.1063/5.0029624
中图分类号
O59 [应用物理学];
学科分类号
摘要
Due to large binding energy and oscillator strength, 2D Ruddlesden-Popper perovskites are promising materials for the realization of room temperature coupled exciton-polaritons. Here, we demonstrate room temperature exciton-polaritons in high-quality exfoliated 2D RPP (BA)(2)(MA)(n-1)PbnI3n+1 (n=3, 4) flakes without the use of external Distributed Bragg Reflectors. By angle-resolved PL spectroscopy, we obtain multi-mode low polariton branches and the Rabi splitting in the range of about 160meV-180meV for n=3 and n=4 flakes. The realization of room temperature exciton-polaritons in 2D RPPs with a large n value provides a potential platform for polaritonic device applications.
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页数:7
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