Orbitally induced string formation in the spin-orbital polarons

被引:36
|
作者
Wohlfeld, Krzysztof [1 ,2 ]
Oles, Andrzej M. [1 ,2 ]
Horsch, Peter [1 ]
机构
[1] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany
[2] Jagiellonian Univ, Marian Smoluchowski Inst Phys, PL-30059 Krakow, Poland
关键词
antiferromagnetic materials; Ising model; lanthanum compounds; localised states; magnetic polarons; magnetic transitions; magnons; spin dynamics; spin-orbit interactions; superexchange interactions; t-J model; METAL-INSULATOR-TRANSITION; T-J-MODEL; PHOTOEMISSION SPECTRA; SINGLE-HOLE; EXCITATIONS; DYNAMICS;
D O I
10.1103/PhysRevB.79.224433
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We study the spectral function of a single hole doped into the ab plane of the Mott insulator LaVO3, with antiferromagnetic (AF) spin order of S=1 spins accompanied by alternating orbital (AO) order of active {d(yz),d(zx)} orbitals. Starting from the respective t-J model, with spin-orbital superexchange and effective three-site hopping terms, we derive the polaron Hamiltonian and show that a hole couples simultaneously to the collective excitations of the AF/AO phase, magnons, and orbitons. Next, we solve this polaron problem using the self-consistent Born approximation and find a stable quasiparticle solution-a spin-orbital polaron. We show that the spin-orbital polaron resembles the orbital polaron found in e(g) systems, as e.g., in K2CuF4 or (to some extent) in LaMnO3, and that the hole may be seen as confined in a stringlike potential. However, the spins also play a crucial role in the formation of this polaron-we explain how the orbital degrees of freedom: (i) confine the spin dynamics acting on the hole as the classical Ising spins and (ii) generate the string potential which is of the joint spin-orbital character. Finally, we discuss the impact of the results presented here on the understanding of the phase diagrams of the lightly doped cubic vanadates.
引用
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页数:17
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