Production of BTX through Catalytic Depolymerization of Lignin

被引：21

作者：

Fan, Ming-hui ^{[1
]}

Deng, Shu-mei ^{[1
]}

Wang, Tie-jun ^{[2
]}

Li, Quan-xin ^{[1
]}

机构：

[1] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Peoples R China

[2] Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China

来源：

CHINESE JOURNAL OF CHEMICAL PHYSICS | 2014年 / 27卷 / 02期

基金：

中国国家自然科学基金;

关键词：

Lignin; Benzene; Toluene; Xylenes; Depolymerization; PYROLYSIS VAPORS; BED REACTOR; AROMATICS; CONVERSION; ZEOLITE; BIOMASS; OIL; HYDRODEOXYGENATION; BIOREFINERIES; VALORIZATION;

D O I：

10.1063/1674-0068/27/02/221-226

中图分类号：

O64 [物理化学（理论化学）、化学物理学]; O56 [分子物理学、原子物理学];

学科分类号：

070203 ; 070304 ; 081704 ; 1406 ;

摘要：

Lignin is the only nature renewable resource which can provide large quantities of aromatic compounds. In the work, transformation of lignin into benzene, toluene, and xylenes (BTX) was investigated over the HZSM-5, HY, and MCM-22 catalysts, and the HZSM-5 catalyst showed the highest carbon yield of BTX. The reaction condition, including temperature, the gas flow rate, and the catalyst/lignin ratio, was also investigated. The carbon yield of BTX reached about 25.3 C-mol% over HZSM-5 catalyst under T=550 degrees C, f (N-2)=300cm(3)/min, and catalyst/lignin ratio of 2.

引用

页码：221 / 226

页数：6

共 50 条

[1] Production of BTX through Catalytic Depolymerization of Lignin
Ming-hui Fan
Shu-mei Deng
Tie-jun Wang
Quan-xin Li
[J]. Chinese Journal of Chemical Physics, 2014, 27 (02) : 97 - 102
[2] Phenolics Production through Catalytic Depolymerization of Alkali Lignin with Metal Chlorides
Zhang, Xinghua
Zhang, Qi
Long, Jinxing
Xu, Ying
Wang, Tiejun
Ma, Longlong
Li, Yuping
[J]. BIORESOURCES, 2014, 9 (02): : 3347 - 3360
[3] Aromatic chemicals production through various heterogeneous catalytic lignin depolymerization processes
Zhang, Shuting
Kruger, Jacob
Katahira, Rui
Beckham, Gregg
[J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2016, 251
[4] Assessing the potential for upscaling the continuous production of lignin oils through reductive catalytic depolymerization
Jusner, Paul
Sridharan, Balaji
Daelemans, Brent
Mukherjee, Agneev
Van Dael, Miet
Polizzi, Viviana
Servaes, Kelly
Elst, Kathy
Vanbroekhoven, Karolien
Feghali, Elias
[J]. Chemical Engineering Journal, 2024, 499
[5] Advances in Catalytic Depolymerization of Lignin
Wan, Zhouyuanye
Zhang, Hongjie
Guo, Yanzhu
Li, Haiming
[J]. CHEMISTRYSELECT, 2022, 7 (40):
[6] Production of phenols from lignin via depolymerization and catalytic cracking
Yoshikawa, Takuya
Yagi, Taichi
Shinohara, Satoshi
Fukunaga, Tetsuya
Nakasaka, Yuta
Tago, Teruoki
Masuda, Takao
[J]. FUEL PROCESSING TECHNOLOGY, 2013, 108 : 69 - 75
[7] Progress in catalytic depolymerization of lignin
Shu, Riyang
Xu, Ying
Zhang, Qi
Ma, Longlong
Wang, Tiejun
[J]. Huagong Xuebao/CIESC Journal, 2016, 67 (11): : 4523 - 4532
[8] Catalytic Depolymerization of Lignin in Supercritical Ethanol
Huang, Xiaoming
Koranyi, Tamas I.
Boot, Michael D.
Hensen, Emiel J. M.
[J]. CHEMSUSCHEM, 2014, 7 (08) : 2276 - 2288
[9] Towards Quantitative Catalytic Lignin Depolymerization
Roberts, Virginia. M.
Stein, Valentin
Reiner, Thomas
Lemonidou, Angeliki
Li, Xuebing
Lercher, Johannes A.
[J]. CHEMISTRY-A EUROPEAN JOURNAL, 2011, 17 (21) : 5939 - 5948
[10] Catalytic Lignin Depolymerization to Aromatic Chemicals
Zhang, Chaofeng
Wang, Feng
[J]. ACCOUNTS OF CHEMICAL RESEARCH, 2020, 53 (02) : 470 - 484

← 1 2 3 4 5 →