Spatial variations and development of land use regression models of oxidative potential in ten European study areas

被引：32

作者：

Jedynska, Aleksandra ^{[1
]}

Hoek, Gerard ^{[2
]}

Wang, Meng ^{[2
,21
]}

Yang, Aileen ^{[2
,20
]}

Eeftens, Marloes ^{[2
,17
,18
]}

Cyrys, Josef ^{[3
,4
]}

Keuken, Menno ^{[1
]}

Ampe, Christophe ^{[5
]}

Beelen, Rob ^{[20
]}

Cesaroni, Giulia

Forastiere, Francesco ^{[6
]}

Cirach, Marta ^{[7
,8
,9
]}

de Hoogh, Kees ^{[10
,17
,18
]}

De Nazelle, Audrey ^{[7
,19
]}

Nystad, Wenche ^{[11
]}

Akhlaghi, Helgah Makarem ^{[1
]}

Declercq, Christophe ^{[12
]}

Stempfelet, Morgane ^{[12
]}

Eriksen, Kirsten T. ^{[13
]}

Dimakopoulou, Konstantina ^{[14
]}

Lanki, Timo ^{[15
]}

Meliefste, Kees ^{[1
]}

Nieuwenhuijsen, Mark ^{[7
,8
,9
]}

Yli-Tuomi, Tarja ^{[15
]}

Raaschou-Nielsen, Ole ^{[13
]}

Janssen, Nicole A. H. ^{[20
]}

Brunekreef, Bert ^{[2
,16
]}

Kooter, Ingeborg M. ^{[1
]}

机构：

[1] TNO, Netherlands Appl Res Org, Utrecht, Netherlands

[2] Univ Utrecht, Inst Risk Assessment Sci, NL-3508 TC Utrecht, Netherlands

[3] German Res Ctr Environm Hlth, Helmholtz Zentrum Munchen, Neuherberg, Germany

[4] Univ Augsburg, Ctr Environm Sci, Augsburg, Germany

[5] AIRPARIF, Paris, France

[6] Lazio Reg Hlth Serv, Dept Epidemiol, Rome, Italy

[7] Ctr Res Environm Epidemiol CREAL, Barcelona, Spain

[8] Hosp del Mar, Res Inst, IMIM, Barcelona, Spain

[9] CIBERESP, Madrid, Spain

[10] Imperial Coll London, Dept Epidemiol & Biostat, MRC PHA Ctr Environm & Hlth, London, England

[11] Norwegian Inst Publ Hlth, Div Epidemiol, Oslo, Norway

[12] French Inst Publ Hlth Surveillance InVS, St Maurice, France

[13] Danish Canc Soc, Res Ctr, Copenhagen, Denmark

[14] Natl & Kapodistrian Univ Athens, Sch Med, Dept Hyg Epidemiol & Med Stat, Athens, Greece

[15] Natl Inst Hlth & Welf THL, Dept Environm Hlth, Kuopio, Finland

[16] Univ Med Ctr Utrecht, Julius Ctr Hlth Sci & Primary Care, Utrecht, Netherlands

[17] Swiss Trop & Publ Hlth Inst, Basel, Switzerland

[18] Univ Basel, Basel, Switzerland

[19] Imperial Coll London, Ctr Environm Policy, London, England

[20] Natl Inst Publ Hlth & Environm RIVM, Bilthoven, Netherlands

[21] Univ Washington, Dept Environm & Occupat Hlth Sci, Seattle, WA 98195 USA

来源：

ATMOSPHERIC ENVIRONMENT | 2017年 / 150卷

关键词：

Oxidative potential; DTT; LUR; PM2.5; Spatial variation; AIRBORNE PARTICULATE MATTER; AIR-POLLUTION EXPOSURE; DITHIOTHREITOL DTT; CHEMICAL-COMPOSITION; ULTRAFINE PARTICLES; REDOX ACTIVITY; SITES; NO2; PM; PAH;

D O I：

10.1016/j.atmosenv.2016.11.029

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Oxidative potential (OP) has been suggested as a health-relevant measure of air pollution. Little information is available about OP spatial variation and the possibility to model its spatial variability. Our aim was to measure the spatial variation of OP within and between 10 European study areas. The second aim was to develop land use regression (LUR) models to explain the measured spatial variation. OP was determined with the dithiothreitol (DTT) assay in ten European study areas. DTT of PM2.5 was measured at 16-40 sites per study area, divided over street, urban and regional background sites. Three two-week samples were taken per site in a one-year period in three different seasons. We developed study-area specific LUR models and a LUR model for all study areas combined to explain the spatial variation of OP. Significant contrasts between study areas in OP were found. OP DTT levels were highest in southern Europe. DTT levels at street sites were on average 1.10 times higher than at urban background locations. In 5 of the 10 study areas LUR models could be developed with a median R-2 of 33%. A combined study area model explained 30% of the measured spatial variability. Overall, LUR models did not explain spatial variation well, possibly due to low levels of OP DTT and a lack of specific predictor variables. (C) 2016 Elsevier Ltd. All rights reserved.

引用

页码：24 / 32

页数：9

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