Three-dimensional sandglass magnet with non-Kramers ions

被引:1
|
作者
Yang, Yan-Xing [1 ]
Wang, Yao [1 ]
Ding, Zhao-Feng [1 ]
Hillier, A. D. [2 ]
Shu, Lei [1 ,3 ,4 ]
机构
[1] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200438, Peoples R China
[2] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX110QX, Oxon, England
[3] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China
[4] Shanghai Res Ctr Quantum Sci, Shanghai 201315, Peoples R China
关键词
SPIN-LIQUID STATE; QUANTUM; ORDER; FIELD;
D O I
10.1103/PhysRevB.105.174418
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Magnetic susceptibility, specific heat, and muon spin relaxation (??SR) measurements have been performed on a synthesized three-dimensional sandglass-type lattice Tm3SbO7, where two inequivalent sets of non-Kramers 2 ) show crystal electrical field effect at different temperature ranges. The existence of an ordered or a glassy state down to 0.1 K in zero field is excluded. The low-energy properties of Tm3SbO7 are dominated by the lowest non-Kramers quasidoublet of Tm3+1 , and the energy splitting is regarded as an intrinsic transverse field. Therefore, the low-temperature paramagnetic phenomenon in Tm3SbO7 is explained by a transverse field Ising model, which is supported by the quantitative simulation of specific heat data. In addition, the perturbation from Tm23+ may play an important role in accounting for the low temperature spin dynamics behavior observed by ??SR.
引用
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页数:7
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