The goal of this paper is to probe phenomenological implications of large fluctuations of quantum geometry in the Planck era, using cosmology of the early universe. For the background (Friedmann, Lemaitre, Robertson, Walker) quantum geometry, we allow ' widely spread' states in which the relative dispersions are as large as 168% in the Planck regime. By introducing suitable methods to overcome the ensuing conceptual and computational issues, we calculate the power spectrum P-R(k) and the spectral index n(s)(k) of primordial curvature perturbations. These results generalize the previous work in loop quantum cosmology which focused on those states which were known to remain sharply peaked throughout the Planck regime. Surprisingly, even though the fluctuations we now consider are large, their presence does not add new features to the final PR(k) and ns(k): within observational error bars, their effect is degenerate with a different freedom in the theory, namely the number of pre-inflationary e-folds N-B between the bounce and the onset of inflation. Therefore, with regard to observational consequences, one can simulate the freedom in the choice of states with large fluctuations in the Planck era using the simpler, sharply peaked states, simply by allowing for different values of N-B.