Deterministic strain-induced arrays of quantum emitters in a two-dimensional semiconductor

被引:386
|
作者
Branny, Artur [1 ]
Kumar, Santosh [1 ]
Proux, Raphael [1 ]
Gerardot, Brian D. [1 ]
机构
[1] Heriot Watt Univ, SUPA, Inst Photon & Quantum Sci, Edinburgh EH14 4AS, Midlothian, Scotland
来源
NATURE COMMUNICATIONS | 2017年 / 8卷
基金
欧洲研究理事会; 英国工程与自然科学研究理事会;
关键词
ATOMICALLY THIN SEMICONDUCTOR; SINGLE-PHOTON EMITTERS; MONOLAYER WSE2; LOCALIZED EXCITONS; BILAYER WSE2; DOTS; CONFINEMENT; EMISSION; LIGHT; WIRES;
D O I
10.1038/ncomms15053
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
An outstanding challenge in quantum photonics is scalability, which requires positioning of single quantum emitters in a deterministic fashion. Site positioning progress has been made in established platforms including defects in diamond and self-assembled quantum dots, albeit often with compromised coherence and optical quality. The emergence of single quantum emitters in layered transition metal dichalcogenide semiconductors offers new opportunities to construct a scalable quantum architecture. Here, using nanoscale strain engineering, we deterministically achieve a two-dimensional lattice of quantum emitters in an atomically thin semiconductor. We create point-like strain perturbations in mono-and bi-layer WSe2 which locally modify the band-gap, leading to efficient funnelling of excitons towards isolated strain-tuned quantum emitters that exhibit high-purity single photon emission. We achieve near unity emitter creation probability and a mean positioning accuracy of 120 +/- 32 nm, which may be improved with further optimization of the nanopillar dimensions.
引用
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页数:7
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