Electrochemical impedance spectroscopy study of thermally grown oxides exhibiting constant phase element behaviour

被引：74
|
作者：
Hamadou, L. [1 ]
Ainouche, L. [1 ]
Kadri, A. [1 ]
Yahia, S. Ait Ali [1 ]
Benbrahim, N. [1 ]
机构：
[1] Univ Mouloud Mammeri Tizi Ouzou, Lab Phys & Chim Mat, Tizi Ouzou 15000, Algeria
来源：
ELECTROCHIMICA ACTA | 2013年 / 113卷
关键词：
Carbon steel; Titanium; EIS; Oxidation; PASSIVE FILMS; SEMICONDUCTING PROPERTIES; RESISTIVITY DISTRIBUTIONS; ELECTRONIC-PROPERTIES; FREQUENCY DISPERSION; CAPACITANCE; MODEL; TITANIUM; STATES; WATER;
D O I：
10.1016/j.electacta.2013.09.054
中图分类号：
O646 [电化学、电解、磁化学];
学科分类号：
081704 ;
摘要：
Thermally grown oxide films on carbon steel and titanium were investigated with electrochemical impedance spectroscopy (EIS). EIS data were analyzed in two different ways: by the analysis of imaginary part of the impedance in the high frequency domain and by the electrical equivalent circuit fitting. Three approaches for estimating effective capacitances from constant phase element have been used in this work: Brug, Hsu-Mansfeld formulas and power-law model. The approaches yield different semiconducting characteristics as well as different oxide layer thicknesses. (C) 2013 Elsevier Ltd. All rights reserved.
引用
收藏
页码：99 / 108
页数：10
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