Radiative Effects of Residential Sector Emissions in China: Sensitivity to Uncertainty in Black Carbon Emissions

被引:6
|
作者
Archer-Nicholls, S. [1 ,2 ]
Lowe, D. [3 ]
Lacey, F. [1 ,3 ]
Kumar, R. [1 ]
Xiao, Q. [4 ]
Liu, Y. [4 ]
Carter, E. [5 ]
Baumgartner, J. [6 ]
Wiedinmyer, C. [1 ,7 ]
机构
[1] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA
[2] Univ Cambridge, Dept Chem, Ctr Atmospher Sci, Cambridge, England
[3] Univ Manchester, Sch Earth Atmospher & Environm Sci, Ctr Atmospher Sci, Manchester, Lancs, England
[4] Tsinghua Univ, Sch Environm, Beijing, Peoples R China
[5] Colorado State Univ, Walter Scott Jr Coll Engn, Ft Collins, CO 80523 USA
[6] McGill Univ, Dept Epidemiol Biostat & Occupat Hlth, Inst Hlth & Social Policy, Montreal, PQ, Canada
[7] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
基金
美国国家科学基金会;
关键词
Aerosols; Black Carbon; Emissions; Cook stoves; Radiative forcing; WRF-Chem; TERM CLIMATE-CHANGE; AIR-POLLUTION; CROP RESIDUE; BROWN CARBON; MIXING-STATE; NEAR-TERM; ANTHROPOGENIC EMISSIONS; MARINE STRATOCUMULUS; WINTER HAZE; AEROSOL;
D O I
10.1029/2018JD030120
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Residential sector emissions of aerosols, primarily from solid fuels burned for cooking and heating purposes, are high in black carbon, a component that absorbs radiation efficiently across a wideband of wavelengths. Mitigation of residential sector emissions has been suggested as a method to rapidly reduce anthropogenic global warming. This study presents model results from a regional model with coupled chemistry, aerosols, and dynamics over an East Asian domain for January 2014 to investigate the radiative effects of residential sector emissions. Model results are evaluated against surface measurements of particulate matter and remote sensing products, comparing well but with a high aerosol optical depth bias over Sichuan and low single scattering albedo over many locations. We calculate effective radiative forcing of residential sector aerosols at the top of the atmosphere of +1.22W/m(2) over Eastern China, +1.04W/m(2) due to shortwave and +0.18W/m(2) due to longwave forcing. We decompose the shortwave forcing into component parts and find the direct radiative effect is the dominant component (+0.79W/m(2)), with a smaller contribution from semidirect effects (+0.54W/m(2)) partly countered by negative indirect effects (-0.29W/m(2)). The effective radiative forcing varies from 0.20 to 1.97W/m(2) across a reasonable range of black carbon to total carbon emission ratios for the residential sector. Overall, this study shows that mitigation of the residential sector is likely a viable method to locally reduce short-term atmospheric warming in China, but efforts are needed to reduce uncertainty in composition of residential sector emissions to be confident in this conclusion.
引用
收藏
页码:5029 / 5044
页数:16
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