Fischer-Tropsch synthesis in a microstructured reactor

被引:101
|
作者
Myrstad, Rune [1 ]
Eri, Sigrid [4 ]
Pfeifer, Peter [2 ]
Rytter, Erling [4 ]
Holmen, Anders [3 ]
机构
[1] SINTEF Mat & Chem, N-7465 Trondheim, Norway
[2] Forschungszentrum Karlsruhe, D-76344 Eggenstein Leopoldshafen, Germany
[3] Norwegian Univ Sci & Technol, N-7491 Trondheim, Norway
[4] StatoilHydro R&D, Res Ctr, N-7005 Trondheim, Norway
关键词
Fischer-Tropsch synthesis; Microstructured reactor; Microchannel reactor; Cobalt; Alumina; DEACTIVATION; CATALYSTS;
D O I
10.1016/j.cattod.2009.07.011
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
A multichannel microstructured packed bed reactor is manufactured. The performance of the microstructured reactor for Fischer-Tropsch synthesis with high activity cobalt/alumina catalysts is studied. For evaluation of the microstructured reactor performance, the results are compared with results obtained in an electrically heated laboratory scale fixed-bed reactor under similar conditions. The catalyst activity and selectivities obtained with undiluted catalyst in the microstructured reactor are similar to results obtained with diluted catalyst in the fixed-bed reactor. The microstructured reactor's capability to operate with high active catalysts at severe conditions without causing temperature runaways and thus increased deactivation of the catalyst is demonstrated. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:S301 / S304
页数:4
相关论文
共 50 条
  • [1] FISCHER-TROPSCH SYNTHESIS GAS CONVERSION REACTOR
    BLANKS, RF
    [J]. CHEMICAL ENGINEERING SCIENCE, 1992, 47 (05) : 959 - 966
  • [2] Fischer-Tropsch Synthesis in a Fixed Bed Reactor
    Moutsoglou, Alex
    Sunkara, Posi Praveen
    [J]. ENERGY & FUELS, 2011, 25 (05) : 2242 - 2257
  • [3] Fischer-Tropsch results and their analysis for reactor synthesis
    Ngwenya, T
    Glasser, D
    Hildebrandt, D
    Coville, N
    Mukoma, P
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2005, 44 (16) : 5987 - 5994
  • [4] Supercritical Adiabatic Reactor for Fischer-Tropsch Synthesis
    Durham, Ed
    Xu, Rui
    Zhang, Sihe
    Eden, Mario R.
    Roberts, Christopher B.
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2013, 52 (09) : 3133 - 3136
  • [5] Modeling of Fischer-Tropsch synthesis in a tubular reactor
    Mazzone, L. C. A.
    Fernandes, F. A. N.
    [J]. LATIN AMERICAN APPLIED RESEARCH, 2006, 36 (03) : 141 - 148
  • [6] Influence of channel geometry on Fischer-Tropsch synthesis in microstructured reactors
    Piermartini, Paolo
    Boeltken, Tim
    Selinsek, Manuel
    Pfeifer, Peter
    [J]. CHEMICAL ENGINEERING JOURNAL, 2017, 313 : 328 - 335
  • [7] FISCHER-TROPSCH REACTOR SELECTION
    FOX, JM
    [J]. CATALYSIS LETTERS, 1990, 7 (1-4) : 281 - 292
  • [8] Microstructured Fischer-Tropsch Reactor Scale-up and Opportunities for Decentralized Application
    Loewert, Marcel
    Hoffmann, Julian
    Piermartini, Paolo
    Selinsek, Manuel
    Dittmeyer, Roland
    Pfeifer, Peter
    [J]. CHEMICAL ENGINEERING & TECHNOLOGY, 2019, 42 (10) : 2202 - 2214
  • [9] An experimental study on a microchannel reactor for Fischer-Tropsch synthesis
    Ying, Xiang
    Zhang, Li
    Xu, Hong
    Ren, Yanlun
    Xuan, Jin
    [J]. INTERNATIONAL CONFERENCE ON APPLIED ENERGY, ICAE2014, 2014, 61 : 1394 - 1397
  • [10] Experimental investigation of Fischer-Tropsch synthesis in a microchannel reactor
    Ying, Xiang
    Zhang, Li
    Xu, Hong
    Luo, Qing
    Zhu, Hongwei
    [J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2015, 249