Quadrupolar and dipolar magnetic order in DyPd3S4:: A neutron scattering and muon spin rotation and relaxation investigation -: art. no. 060407

被引:8
|
作者
Keller, L [1 ]
Pomjakushin, V
Conder, K
Schenck, A
机构
[1] Swiss Fed Inst Technol, Neutron Scattering Lab, CH-5232 Villigen, Switzerland
[2] PSI, CH-5232 Villigen, Switzerland
[3] Swiss Fed Inst Technol, Inst Particle Phys, CH-5232 Villigen, Switzerland
关键词
D O I
10.1103/PhysRevB.70.060407
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The quadrupolar and dipolar magnetic phases in polycrystalline DyPd3S4 have been investigated by neutron scattering and muon spin rotation/relaxation (muSR) technique. The transition from paramagnetic to antiferroquadrupolar state at T-Q=3.4 K as well as two successive dipolar magnetic phase transitions at T(N1)approximate to1 K and T(N2)approximate to0.8 K are evidenced by anomalies in the observed relaxation rates in the zero-field muSR measurements. In addition, measurements in longitudinal external magnetic field showed clear evidence for field-induced dipolar magnetic moments below T-Q. In inelastic neutron scattering measurements the transition to an ordered lattice of the Dy quadrupole moments at T-Q is observed by a temperature dependent splitting of the ground-state crystal-field multiplet below T-Q. Neutron diffraction revealed the induced magnetic structure in the quadrupolar phase of DyPd3S4 to be of the canted antiferromagnetic type with a canting angle close to perpendicular, similar to the spontaneous zero-field magnetic structures below 1 K.
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页码:060407 / 1
页数:4
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