Robust Metal-Organic Framework Containing Benzoselenadiazole for Highly Efficient Aerobic Cross-dehydrogenative Coupling Reactions under Visible Light

被引：70
|
作者：
Zhang, Wen-Qiang [1 ]
Li, Qiu-Yan [1 ]
Zhang, Quan [2 ]
Lu, Yingqiao [1 ]
Lu, Han [1 ]
Wang, Wenguang [3 ]
Zhao, Xinsheng [4 ]
Wang, Xiao-Jun [1 ]
机构：
[1] Jiangsu Normal Univ, Sch Chem & Chem Engn, Jiangsu Key Lab Green Synthet Chem Funct Mat, Xuzhou 221116, Peoples R China
[2] Jiangnan Univ, Sch Biotechnol, Key Lab Carbohydrate Chem & Biotechnol, Minist Educ, Wuxi 214122, Peoples R China
[3] Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China
[4] Jiangsu Normal Univ, Sch Phys & Elect Engn, Xuzhou 221116, Peoples R China
来源：
INORGANIC CHEMISTRY | 2016年 / 55卷 / 03期
关键词：
C-H FUNCTIONALIZATION; PHOTOREDOX CATALYSIS; ARYLBORONIC ACIDS; BONDS; WATER; VERSATILE; PHOTOCATALYSIS; OXIDATION; STRATEGY; COMPLEX;
D O I：
10.1021/acs.inorgchem.5b02626
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A zirconium(IV)-based UiO-topological metal-organic framework (UiO-68Se) containing benzoselenadiazole was synthesized by an approach of the mixed dicarboxylate struts, which show highly efficient and recycalable photocatalytic activity for aerobic cross-dehydrogenative coupling reactions between tertiary amines and various carbon nucleophiles under visible-light irradiation.
引用
收藏
页码：1005 / 1007
页数：3
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