A novel method to assay special nuclear materials by measuring prompt neutrons from polarized photofission

A novel method of measuring the enrichment of special nuclear material is presented. Recent photofission measurements using a linearly polarized gamma-ray beam were performed on samples of Th-232, U-233,U-235,U-238, Np-237, and Pu-239,Pu-240. Prompt neutron polarization asymmetries, defined to be the difference in the prompt neutron yields parallel and perpendicular to the plane of beam polarization divided by their sum, were measured. It was discovered that the prompt neutron polarization asymmetries differed significantly depending on the sample. Prompt neutrons from photofission of even-even (non-fissile) targets had significant polarization asymmetries (similar to 0.2 to 0.5), while those from odd-A (generally fissile) targets had polarization asymmetries close to zero. This difference in the polarization asymmetries could be exploited to measure the fissile versus non-fissile content of special nuclear materials, and potentially to detect the presence of fissile material during active interrogation. The proposed technique, its expected performance, and its potential applicability are discussed. (C) 2014 Elsevier B.V. All rights reserved