Bottom-Up Emission Inventory and Its Spatio-Temporal Distribution from Paved Road Dust Based on Field Investigation: A Case Study of Harbin, Northeast China

Road dust is one of the primary sources of particulate matter which has implications for air quality, climate and health. With the aim of characterizing the emissions, in this study, a bottom-up approach of county level emission inventory from paved road dust based on field investigation was developed. An inventory of high-resolution paved road dust (PRD) emissions by monthly and spatial allocation at 1 km x 1 km resolution in Harbin in 2016 was compiled using accessible county level, seasonal data and local parameters based on field investigation to increase temporal-spatial resolution. The results demonstrated the total PRD emissions of TSP, PM10, and PM2.5 in Harbin were 270,207 t, 54,597 t, 14,059 t, respectively. The temporal variation trends of pollutant emissions from PRD was consistent with the characteristics of precipitation, with lower emissions in winter and summer, and higher emissions in spring and autumn. The spatial allocation of emissions has a strong association with Harbin's road network, mainly concentrating in the central urban area compared to the surrounding counties. Through scenario analysis, positive control measures were essential and effective for PRD pollution. The inventory developed in this study reflected the level of fugitive dust on paved road in Harbin, and it could reduce particulate matter pollution with the development of mitigation strategies and could comply with air quality modelling requirements, especially in the frigid region of northeastern China.