Greener processes in the preparation of thin film nanocomposite membranes with diverse metal-organic frameworks for organic solvent nanofiltration

被引：43
|
作者：
Paseta, Lorena [1 ,2 ]
Navarro, Marta [1 ,2 ]
Coronas, Joaquin [1 ,2 ,3 ]
Tellez, Carlos [1 ,2 ,3 ]
机构：
[1] Univ Zaragoza, INA, Zaragoza 50018, Spain
[2] Univ Zaragoza, Chem & Environm Engn Dept, Zaragoza 50018, Spain
[3] Univ Zaragoza, ICMA, CSIC, Zaragoza 50018, Spain
来源：
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY | 2019年 / 77卷
关键词：
Greener preparation process; Organic solvent nanofiltration; Thin film nanocomposite; Metal-organic frameworks; COMPOSITE REVERSE-OSMOSIS; SOLUBILITY PARAMETERS; TIO2; NANOPARTICLES; DRINKING-WATER; TFN MEMBRANE; PERFORMANCE; POLYMERIZATION; ENCAPSULATION; MIL-101(CR); FABRICATION;
D O I：
10.1016/j.jiec.2019.04.057
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The toxic solvent dimethylformamide has been replaced by the greener dimethylsulfoxide in the casting and activation processes for the preparation of thin film composite (TFC) membranes. This methodology has been validated with the use of MOFs ZIF-8, ZIF-93 and UIO-66 as fillers for thin-film nanocomposite (TFN) membranes. These membranes were successfully applied in the organic solvent nanofiltration of sunset yellow (SY) in methanol obtaining the highest permeance when UiO-66 and ZIF-93 were used with a value of 11 Lm(-2)h(-1) bars. The permeance improvements are related to the MOF porosity, polyamide-MOF layer thickness and the hydrophilic/hydrophobic character of the membrane. (C) 2019 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码：344 / 354
页数：11
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