Efficient removal of nitrobenzene and concomitant electricity production by single-chamber microbial fuel cells with activated carbon air-cathode

被引:27
|
作者
Zhang, Enren [1 ]
Wang, Feng [1 ]
Zhai, Wenjing [1 ]
Scott, Keith [2 ]
Wang, Xu [3 ]
Diao, Guowang [1 ]
机构
[1] Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Jiangsu, Peoples R China
[2] Newcastle Univ, Sch Chem Engn & Adv Mat, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England
[3] Wuhan Univ, Sch Resource & Environm Sci, Wuhan 430079, Peoples R China
基金
中国国家自然科学基金;
关键词
Nitrobenzene removal; Microbial fuel cells; Activated carbon air-cathode; Bio-electrochemical system; PHOTOCATALYTIC DEGRADATION; ANODIC-OXIDATION; REDUCTION; GENERATION; PERFORMANCE; BIODEGRADATION; COMMUNITY; CATALYSTS; ELECTRODE; MEMBRANE;
D O I
10.1016/j.biortech.2017.01.009
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
Single-chamber microbial fuel cells (S-MFCs) with bio-anodes and activated carbon (AC) air-cathodes showed high nitrobenzene (NB) tolerance and NB removal with concomitant electricity production. The maximum power over 25 W m(-3) could be obtained when S-MFCs were operated in the NB loading range of 1.2-6.2 mol m(-3) d(-1), and stable electricity production over 13.7 W m(-3) could be produced in a NB loading range of 1.2-14.7 mol m(-3) d(-1). The present S-MFCs exhibited high NB removal performance with NB removal efficiency over 97% even when the NB loading rate was increased to 17.2 mol m(-3) d(-1). The potential NB reduced product (i.e. aniline) could also be effectively removed from influents. The findings in this study means that single-chamber MFCs assembled with pre-enriched bio-anodes and AC aircathodes could be developed as effective bio-electrochemical systems to remove NB from wastewaters and to harvest energy instead of consuming energy. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:111 / 118
页数:8
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