Bismuth sulfide: A high-capacity anode for sodium-ion batteries

被引：119
|
作者：
Sun, Wenping [1 ]
Rui, Xianhong [2 ,4 ]
Zhang, Dan [1 ,3 ]
Jiang, Yinzhu [3 ]
Sun, Ziqi [5 ]
Liu, Huakun [1 ]
Dou, Shixue [1 ]
机构：
[1] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia
[2] Anhui Univ Technol, Sch Energy & Environm, Maanshan 243002, Anhui, Peoples R China
[3] Zhejiang Univ, State Key Lab Silicon Mat, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China
[4] Nankai Univ, Minist Educ, Key Lab Adv Energy Mat, Tianjin 300071, Peoples R China
[5] Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4000, Australia
来源：
JOURNAL OF POWER SOURCES | 2016年 / 309卷
基金：
中国国家自然科学基金;
关键词：
Bismuth sulfide; Nanorods; Anode; Sodium-ion batteries; HIGH-PERFORMANCE ANODE; CARBON-COATED NA3V2(PO4)(3); NEGATIVE ELECTRODES; HARD-CARBON; STORAGE; NANOSHEETS; LITHIUM; OXIDE; NANOCOMPOSITES; SB;
D O I：
10.1016/j.jpowsour.2016.01.092
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Exploring high-performance anode materials is currently one of the most urgent issues towards practical sodium-ion batteries (SIBs). In this work, Bi2S3 is demonstrated to be a high-capacity anode for SIBs for the first time. The specific capacity of Bi2S3 nanorods achieves up to 658 and 264 mAh g(-1) at a current density of 100 and 2000 mA g(-1), respectively. A full cell with Na3V2(PO4)(3)-based cathode is also assembled as a proof of concept and delivers 340 mAh g(-1) at 100 mA g(-1). The sodium storage mechanism of Bi2S3 is investigated by ex-situ XRD coupled with high-resolution TEM (HRTEM), and it is found that sodium storage is achieved by a combined conversion-intercalation mechanism. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码：135 / 140
页数：6
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