Experiment and Modeling Studies on Absorption of CO2 by Dilute Ammonia in Rotating Packed Bed

被引:14
|
作者
Kang, Jia-Lin [1 ]
Luo, Zhen-Jie [1 ]
Liu, Jia-Lin [1 ]
Sun, Kai [2 ]
Wong, David Shan-Hill [1 ]
Jang, Shi-Shang [1 ]
Tan, Chung-Sung [1 ]
Shen, Jui-Fu [3 ]
机构
[1] Natl Tsing Hua Univ, Dept Chem Engn, Hsinchu, Taiwan
[2] Qilu Univ Technol, Dept Automat, Jinan, Shandong, Peoples R China
[3] China Steel Corp, New Mat Res & Dev Dept, Kaohsiung, Taiwan
关键词
rotating packed bed; packed bed; ammonia; carbon dioxide; CARBON-DIOXIDE; CAPTURE; GAS; MONOETHANOLAMINE; PIPERAZINE;
D O I
10.1016/j.egypro.2014.11.139
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
This study presented experimental data of packed bed and rotating packed bed adsorption of carbon dioxide by dilute aqueous ammonia solutions. The heights of transfer units of packed bed were found to be 0.35 to 1.96 m; while the heights of a transfer unit of the rotating packed bed were in the range 0.08 to 0.40 m. Predictive models of the two processes were developed (model details and implications discussed elsewhere) based on the same set of thermodynamic and kinetic data for carbon dioxide into dilute aqueous ammonia solutions and existing mass transfer correlations for packed bed and rotating packed bed. The average absolute deviations between model predictions and experiments were found to be 9.4% for rotating packed bed data and 12% pack bed data. (C) 2014 The Authors. Published by Elsevier Ltd.
引用
收藏
页码:1308 / 1313
页数:6
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