The Chemistry and Properties of Energetic Materials Bearing [1,2,4]Triazolo[4,3-b][1,2,4,5]tetrazine Fused Rings

被引：22

作者：

Wang, Guilong ^{[1
]}

Lu, Tian ^{[1
]}

Fan, Guijuan ^{[2
]}

Li, Chengqiu ^{[1
]}

Yin, Hongquan ^{[1
]}

Chen, Fu-Xue ^{[1
]}

机构：

[1] Beijing Inst Technol, Sch Chem & Chem Engn, 5 South Zhongguancun St, Beijing 100081, Peoples R China

[2] CAEP, Inst Chem Mat, Mianyang 621050, Peoples R China

来源：

CHEMISTRY-AN ASIAN JOURNAL | 2018年 / 13卷 / 23期

关键词：

1,2,4]triazolo[4,3-b][1,2,4,5]tetrazine; energetic materials; fused rings; nitration; synthesis; HIGH-NITROGEN; LASER INITIATION; HIGH-DENSITY; IONIC SALTS;

D O I：

10.1002/asia.201801145

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Treatment of heterocyclic amines featuring fused rings of [1,2,4]triazolo[4,3-b][1,2,4,5]tetrazine with fuming HNO3/P2O5 leads to six fully characterized explosives through multiple nitration and reduction or oxidation mechanism. Thus, 4-nitro-N-(3-nitro[1,2,4]triazolo[4,3-b][1,2,4,5]tetrazin-6-yl)-1,2,5-oxadiazol-3-amine (3 b, TTDNF) showed high performance (D=9180 m s(-1), P=36.7 GPa) and low impact sensitivity (IS>40 J) while N-([1,2,4]triazolo[4,3-b][1,2,4,5]tetrazin-6-yl)-3-nitro-1,2,4-oxadiazol-5-amine (4 a, TTNOA) exhibited a potential cast explosive component with low melting point at 88.2 degrees C and high onset decomposition temperature at 226.2 degrees C.

引用

页码：3718 / 3722

页数：5

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