Plasmonic Wood for High-Efficiency Solar Steam Generation

被引:760
|
作者
Zhu, Mingwei [1 ,2 ,3 ]
Li, Yiju [1 ]
Chen, Fengjuan [1 ]
Zhu, Xueyi [2 ,3 ]
Dai, Jiaqi [1 ]
Li, Yongfeng [1 ]
Yang, Zhi [4 ]
Yan, Xuejun [2 ,3 ]
Song, Jianwei [1 ]
Wang, Yanbin [1 ]
Hitz, Emily [1 ]
Luo, Wei [1 ]
Lu, Minhui [2 ,3 ]
Yang, Bao [4 ]
Hu, Liangbing [1 ]
机构
[1] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA
[2] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China
[3] Nanjing Univ, Coll Engn & Appl Sci, Nanjing 210093, Jiangsu, Peoples R China
[4] Univ Maryland, Dept Mech Engn, College Pk, MD 20742 USA
关键词
high absorption; natural wood; plasmonic; solar energy; solar steam generation; WASTE-WATER; TRANSPARENT; GRAPHENE; DESALINATION; PAPER;
D O I
10.1002/aenm.201701028
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Plasmonic metal nanoparticles are a category of plasmonic materials that can efficiently convert light into heat under illumination, which can be applied in the field of solar steam generation. Here, this study designs a novel type of plasmonic material, which is made by uniformly decorating fine metal nanoparticles into the 3D mesoporous matrix of natural wood (plasmonic wood). The plasmonic wood exhibits high light absorption ability (approximate to 99%) over a broad wavelength range from 200 to 2500 nm due to the plasmonic effect of metal nanoparticles and the waveguide effect of microchannels in the wood matrix. The 3D mesoporous wood with numerous low-tortuosity microchannels and nanochannels can transport water up from the bottom of the device effectively due to the capillary effect. As a result, the 3D aligned porous architecture can achieve a high solar conversion efficiency of 85% under ten-sun illumination (10 kW m(-2)). The plasmonic wood also exhibits superior stability for solar steam generation, without any degradation after being evaluated for 144 h. Its high conversion efficiency and excellent cycling stability demonstrate the potential of newly developed plasmonic wood to solar energy-based water desalination.
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页数:7
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