Single-atom site catalysts supported on two-dimensional materials for energy applications

被引:40
|
作者
Xu, Qi [1 ]
Zhang, Jian [1 ]
Wang, Dingsheng [1 ]
Li, Yadong [1 ]
机构
[1] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
Single-atom site catalysts; Two-dimensional materials; Synthesis; Characterization; Energy applications; HIGH-DENSITY; EVOLUTION REACTION; OXYGEN EVOLUTION; DOPED GRAPHENE; REDUCTION; RU; ELECTROCATALYST; PHOTOCATALYST; FRAMEWORK; CARBON;
D O I
10.1016/j.cclet.2021.05.032
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Single-atom site catalysts (SACs) and two-dimensional materials (2DM) have gradually become two hot topics in catalysis over the past decades. Their combination with each other can further endow the derived SACs with extraordinary properties such as high loading, identical active sites, uniform coordination environment, distinctive metal-support interaction, and enhanced catalytic activities. In this review, we highlight the recent development in this specific research topic according to the types of substrates and focus on their applications in energy conversion field. Additionally, we also make a brief introduction to the synthesis and characterization methods for SACs supported on 2DM (SACs/2DM). Finally, the challenges and perspectives are summarized based on the current development status. It is believed that this work will make contributions to the rational design and fabrication of novel SACs/2DM, promoting their practical energy applications in the future. (C) 2021 Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences.
引用
收藏
页码:3771 / 3781
页数:11
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