CuO/g-C3N4 nanocomposite as promising photocatalyst for photoelectrochemical water splitting

被引:65
|
作者
Ragupathi, Veena [1 ]
Raja, M. Anthony [1 ]
Panigrahi, Puspamitra [1 ]
Subramaniam, N. Ganapathi [2 ]
机构
[1] Hindustan Inst Technol & Sci HITS, Clean Energy & Nano Convergence CENCON, Chennai 603103, Tamil Nadu, India
[2] Dongguk Univ, Quantum Funct Semicond Res Ctr, Seoul, South Korea
来源
OPTIK | 2020年 / 208卷
关键词
CuO/g-C3N4; nanocomposite; Photoelectrode; Photocatalyst; Photoelectrochemical (PEC) water splitting; Co-precipitation method;
D O I
10.1016/j.ijleo.2020.164569
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
CuO/g-C3N4 nanocomposite photocatalyst has been synthesized by co-precipitation method and analyzed its performance in the photoelectrochemical water splitting application. X-ray diffraction analyses and Raman measurement confirms the presence of CuO. Scanning electron microscope image shows rod shape morphology. The CuO/g-C3N4 nanocomposite exhibit the wide range of visible light absorbance and the bandgap of the material is 1.64 eV. Room temperature photoluminescence measurement reveals the presence of CuO charge transfer emission and LUMO - HUMO transition of g-C3N4. The CuO/g-C3N4 composite shows improved photocatalytic water splitting under visible light illumination. This could be attributed to the higher visible light absorbance and reduction in the recombination rate. The CuO/g-C3N4 nanocomposite electrode shows a highly stable photocurrent response.
引用
收藏
页数:5
相关论文
共 50 条
  • [1] g-C3N4/SnS2 Heterostructure: a Promising Water Splitting Photocatalyst
    Chen, Shao-hua
    Wang, Jia-jun
    Huang, Jing
    Li, Qun-xiang
    [J]. CHINESE JOURNAL OF CHEMICAL PHYSICS, 2017, 30 (01) : 36 - 42
  • [2] The g-C3N4/C2N Nanocomposite: A g-C3N4-Based Water-Splitting Photocatalyst with Enhanced Energy Efficiency
    Wang, Huimin
    Li, Xingxing
    Yang, Jinlong
    [J]. CHEMPHYSCHEM, 2016, 17 (13) : 2100 - 2104
  • [3] Graphitic carbon nitride (g-C3N4)-based nanosized heteroarrays: Promising materials for photoelectrochemical water splitting
    Wang, Liqun
    Si, Wenping
    Tong, Yueyu
    Hou, Feng
    Pergolesi, Daniele
    Hou, Jungang
    Lippert, Thomas
    Dou, Shi Xue
    Liang, Ji
    [J]. CARBON ENERGY, 2020, 2 (02) : 223 - 250
  • [4] One-pot microwave synthesis of hierarchical C-doped CuO dandelions/g-C3N4 nanocomposite with enhanced photostability for photoelectrochemical water splitting
    Hosseini, Seyed Morteza H.
    Moakhar, Roozbeh Siavash
    Soleimani, Foad
    Sadrnezhaad, Sayed Khatiboleslam
    Masudy-Panah, Saeid
    Katal, Reza
    Seza, Ashkan
    Ghane, Navid
    Ramakrishna, Seeram
    [J]. APPLIED SURFACE SCIENCE, 2020, 530
  • [5] Recent Progress in Doped g-C3N4 Photocatalyst for Solar Water Splitting: A Review
    Yang, Yilong
    Niu, Wantong
    Dang, Liyun
    Mao, Yanli
    Wu, Junshu
    Xu, Kaidong
    [J]. FRONTIERS IN CHEMISTRY, 2022, 10
  • [6] A ternary g-C3N4/Pt/ZnO photoanode for efficient photoelectrochemical water splitting
    Xiao, Jingran
    Zhang, Xiaoli
    Li, Yongdan
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2015, 40 (30) : 9080 - 9087
  • [7] Bifunctional Co3O4/g-C3N4 Hetrostructures for Photoelectrochemical Water Splitting
    Shabbir, Syeda Ammara
    Ali, Iqra
    Haris, Muhammad
    Latif, Hamid
    Sabah, Aneeqa
    Alshomrany, Ali S.
    Bakkour, Youssef
    [J]. ACS OMEGA, 2024, 9 (19): : 21450 - 21458
  • [8] Multifarious function layers photoanode based on g-C3N4 for photoelectrochemical water splitting
    Liu, Zhifeng
    Lu, Xue
    [J]. CHINESE JOURNAL OF CATALYSIS, 2018, 39 (09) : 1527 - 1533
  • [9] Novel framework g-C3N4 film as efficient photoanode for photoelectrochemical water splitting
    Lu, Xue
    Liu, Zhifeng
    Li, Junwei
    Zhang, Jing
    Guo, Zhengang
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 209 : 657 - 662
  • [10] A g-C3N4/WO3 photoanode with exceptional ability for photoelectrochemical water splitting
    Li, Haibo
    Zhao, Fengyi
    Zhang, Jincheng
    Luo, Lei
    Xiao, Xujing
    Huang, Yongchao
    Ji, Hongbing
    Tong, Yexiang
    [J]. MATERIALS CHEMISTRY FRONTIERS, 2017, 1 (02) : 338 - 342