We demonstrate a canted magnetization of biatomic zigzag Co chains grown on the (5 x 1) reconstructed Ir(001) surface using density functional theory (DFT) calculations and spin-polarized scanning tunneling microscopy (SP-STM) experiments. It is observed by STM that biatomic Co chains grow in three different structural configurations. Our DFT calculations show that they are all in a ferromagnetic (FM) state. Two chain types possess high symmetry due to two equivalent atomic strands and an easy magnetization direction that is along one of the principal crystallographic axes. The easy magnetization axis of the zigzag Co chains is canted away from the surface normal by an angle of 33 degrees. This giant effect is caused by the broken chain symmetry on the substrate in combination with the strong spin-orbit coupling of Ir. SP-STM measurements confirm the stable FM order of the zigzag chains with a canted magnetization.
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Department of Physics, Princeton University, Princeton, 08544, NJ
Department of Applied Physics, Stanford University, Stanford, 94305, CADepartment of Physics, Princeton University, Princeton, 08544, NJ
Liang T.
Hsieh T.H.
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Department of Physics, Massachusetts Institute of Technology, Cambridge, 02139, MA
Kavli Institute for Theoretical Physics, University of California, Santa Barbara, 93106, CADepartment of Physics, Princeton University, Princeton, 08544, NJ
Hsieh T.H.
Ishikawa J.J.
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Institute for Solid State Physics, University of Tokyo, KashiwaDepartment of Physics, Princeton University, Princeton, 08544, NJ
Ishikawa J.J.
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Nakatsuji S.
Fu L.
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Department of Physics, Massachusetts Institute of Technology, Cambridge, 02139, MADepartment of Physics, Princeton University, Princeton, 08544, NJ
Fu L.
Ong N.P.
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Department of Physics, Princeton University, Princeton, 08544, NJDepartment of Physics, Princeton University, Princeton, 08544, NJ
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Princeton Univ, Dept Phys, Princeton, NJ 08544 USA
Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA
Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USAPrinceton Univ, Dept Phys, Princeton, NJ 08544 USA
Liang, Tian
Hsieh, Timothy H.
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MIT, Dept Phys, Cambridge, MA 02139 USA
Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA
Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USAPrinceton Univ, Dept Phys, Princeton, NJ 08544 USA
Hsieh, Timothy H.
Ishikawa, Jun J.
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Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, JapanPrinceton Univ, Dept Phys, Princeton, NJ 08544 USA
Ishikawa, Jun J.
Nakatsuji, Satoru
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Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan
Japan Sci & Technol Agcy JST, CREST, 4-1-8 Honcho Kawaguchi, Saitama 3320012, JapanPrinceton Univ, Dept Phys, Princeton, NJ 08544 USA
Nakatsuji, Satoru
Fu, Liang
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MIT, Dept Phys, Cambridge, MA 02139 USAPrinceton Univ, Dept Phys, Princeton, NJ 08544 USA
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Xi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R ChinaXi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R China
Hou, W. S.
Dong, M. Q.
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Xi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R ChinaXi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R China
Dong, M. Q.
Zhang, X.
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Xian Univ, Coll Mech & Mat Engn, Shaanxi Key Lab Surface Engn & Remfg, Xian 710065, Peoples R ChinaXi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R China
Zhang, X.
Guo, Zhi-Xin
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Xi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R ChinaXi An Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R China