Hydrogen Production Coupled to Hydrocarbon Oxygenation from Photocatalytic Water Splitting

被引：45
|
作者：
Singh, Wangkheimayum Marjit [1 ]
Pegram, Derek [1 ]
Duan, Haifeng [1 ]
Kalita, Diganta [1 ]
Simone, Paul [1 ]
Emmert, Gary L. [1 ]
Zhao, Xuan [1 ]
机构：
[1] Univ Memphis, Dept Chem, Memphis, TN 38152 USA
来源：
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2012年 / 51卷 / 07期
基金：
美国国家科学基金会;
关键词：
hydrocarbons; hydrogen production; photocatalysis; water splitting; H-2; PRODUCTION; MOLECULAR ELECTROCATALYSTS; GENERATING HYDROGEN; FUNCTIONAL MODELS; PHOTOSYSTEM-II; ACTIVE-SITE; COMPLEXES; COBALT; OXIDATION; REDUCTION;
D O I：
10.1002/anie.201106494
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
On the sunny side: A homogeneous system for H 2 production and hydrocarbon oxidation was developed in the absence of any sacrificial reagent. This system consists of [Ru(TPA)(H 2O) 2] 2+ and [Fe 3(CO) 12] as catalysts and [Ru(bpy) 3] 2+ and [Ir(bpy)(ppy) 2] + as photosensitizers (PS). Water is the oxygen source as well as the source for H 2 formation (see picture; Sub=organic substrate). Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码：1653 / 1656
页数：4
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