Geminate charge recombination with distance-dependent intrinsic reaction rate: Escape probability and its electric field effect

被引：21

作者：

Wojcik, M

Tachiya, M

机构：

[1] Tech Univ Lodz, Inst Appl Radiat Chem, PL-93590 Lodz, Poland

[2] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058565, Japan

来源：

RADIATION PHYSICS AND CHEMISTRY | 2005年 / 74卷 / 3-4期

关键词：

D O I：

10.1016/j.radphyschem.2005.04.005

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We calculate the electric field dependence of the probability of escape from geminate recombination in the case of a finite, distance-dependent intrinsic reaction rate. We solve a partial differential equation for the escape probability using a numerical method. We assess the role of finite-reactivity effects in geminate recombination and discuss their possible consequences for interpretation of experimental data. (C) 2005 Elsevier Ltd. All rights reserved.

引用

页码：132 / 138

页数：7

共 5 条

[1] Kinetics of Distance-Dependent Recombination between Geminate Charge Carriers by Diffusion under Coulomb Interaction
Suzuki, Yohichi
Furube, Akihiro
Singh, Rupashree Balia
Matsuzaki, Hiroyuki
Minegishi, Tsutomu
Hisatomi, Takashi
Domen, Kazunari
Seki, Kazuhiko
JOURNAL OF PHYSICAL CHEMISTRY C, 2015, 119 (10): : 5364 - 5373
[2] INFLUENCE OF FRACTAL GEOMETRY ON GEMINATE ESCAPE PROBABILITY, MEAN RECOMBINATION TIME, AND HOMOGENEOUS REACTION-RATE
MOZUMDER, A
JOURNAL OF CHEMICAL PHYSICS, 1990, 92 (02): : 1015 - 1020
[3] Electron-ion recombination in nuclear recoils tracks in nonpolar liquids. Calculation of the effect of external electric field on the escape probability
Mateja, Piotr
Wojcik, Mariusz
RADIATION PHYSICS AND CHEMISTRY, 2016, 124 : 2 - 6
[4] THE EFFECT OF AN APPLIED ELECTRIC-FIELD ON THE CHARGE RECOMBINATION KINETICS IN REACTION CENTERS RECONSTITUTED IN PLANAR LIPID BILAYERS
GOPHER, A
BLATT, Y
SCHONFELD, M
OKAMURA, MY
FEHER, G
MONTAL, M
BIOPHYSICAL JOURNAL, 1985, 48 (02) : 311 - 320
[5] ELECTRIC-FIELD MODULATION OF ELECTRON-TRANSFER REACTION-RATES IN ISOTROPIC SYSTEMS - LONG-DISTANCE CHARGE RECOMBINATION IN PHOTOSYNTHETIC REACTION CENTERS
FRANZEN, S
GOLDSTEIN, RF
BOXER, SG
JOURNAL OF PHYSICAL CHEMISTRY, 1990, 94 (12): : 5135 - 5149

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