This study estimated the grass alpha, gross beta, K-40, Tl-208, Ac-228 and Bi-214 activities in the sea and subsoil brines of two salt works at Vepalodai and Sahupuram in Tuticorin District, Tamil Nadu, India. It was observed that the sea brine of at Vepalodai, the gross alpha activity in the brine varied from 0.0009 to 0.0033 Bq L-1 and the gross beta activity varied from 0.0194 to 4.0405 Bq L-1. At the subsoil brine of Sahupuram, the corresponding values varied from below detection limit (BDL) to 0.0032 and 0.0114 to 3.0352 Bq L-1. K-40 activity was found to increase, source to bittern, viz., 4.006 to 221.006, at Veplodai and 3.247 to 204.462 Bq L-1 at Sahupuram. The activity of the sea brine was higher than that of the sub-soil brine. The gross alpha and beta activities were increasing at subsequent stages of production due to the concentration of brine. The sediments collected at different stages showed gross alpha activity varying from 42.0 to 362.0 Bq kg(-1), gross beta activity varying from 1998 to 2498 Bq kg(-1). Tl-208, Ac-228 activities varied from 111.2 to 151.2 Bq kg(-1) and 40.1 to 73.4 Bq kg(-1). The corresponding values for Sahupuram salt works were 10.2 to 98.7, 1298 to 1548, 137.4 to 175.8 and 33.8 to 55.3 Bq kg(-1) for gross alpha, gross beta, Tl-208, Ac-228, respectively. The analysis of the common salt from Vepalodai showed 14.4,107, 12.42, 13.10 and 3.8 Bq kg(-1) of gross alpha, gross beta, Tl-208, Ac-228 and Bi-214, respectively and that from sub soil brine of Sahupuram showed 8.7, 24.6, 7.4, 9.46 and 3.4 Bq kg(-1). This study shows that the radioactivity in common salt is within the limit.