High-Conductivity, Flexible and Transparent PEDOT:PSS Electrodes for High Performance Semi-Transparent Supercapacitors

被引:56
|
作者
Song, Jiaxing [1 ]
Ma, Guoqiang [2 ]
Qin, Fei [3 ,4 ]
Hu, Lin [1 ]
Luo, Bangwu [3 ,4 ]
Liu, Tiefeng [3 ,4 ]
Yin, Xinxing [1 ]
Su, Zhen [1 ]
Zeng, Zhaobing [1 ]
Jiang, Youyu [3 ,4 ]
Wang, Guannan [5 ,6 ]
Li, Zaifang [1 ]
机构
[1] Jiaxing Univ, China Australia Inst Adv Mat & Mfg IAMM, Jiaxing 314001, Peoples R China
[2] Wuyi Univ, Sch Appl Phys & Mat, Jiangmen 529020, Peoples R China
[3] Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430074, Peoples R China
[4] Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan 430074, Peoples R China
[5] Jining Med Univ, Coll Biomed Engn, Jining 272067, Peoples R China
[6] Jining Med Univ, Key Lab Med Funct Nanomat, Jining 272067, Peoples R China
基金
中国国家自然科学基金;
关键词
conducting polymer; PEDOT:PSS; high conductivity; semi-transparent supercapacitors; high power density; CARBON NANOTUBE; FILMS; POLYMER; GRAPHENE; LAYER;
D O I
10.3390/polym12020450
中图分类号
O63 [高分子化学(高聚物)];
学科分类号
070305 ; 080501 ; 081704 ;
摘要
Herein, we report a flexible high-conductivity transparent electrode (denoted as S-PH1000), based on conducting polymer poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS), and itsapplication to flexible semi-transparentsupercapacitors. A high conductivity of 2673 S/cm was achieved for the S-PH1000 electrode on flexible plastic substrates via a H2SO4 treatment with an optimized concentration of 80 wt.%. This is among the top electrical conductivities of PEDOT:PSS films processed on flexible substrates. As for the electrochemical properties,a high specific capacitance of 161F/g was obtained from the S-PH1000 electrode at a current density of 1 A/g. Excitingly, a specific capacitance of 121 F/g was retained even when the current density increased to 100 A/g, which demonstrates the high-rate property of this electrode. Flexible semi-transparent supercapacitors based on these electrodes demonstrate high transparency, over 60%, at 550 nm. A high power density value, over 19,200 W/kg,and energy density, over 3.40 Wh/kg, was achieved. The semi-transparent flexible supercapacitor was successfully applied topower a light-emitting diode.
引用
收藏
页数:10
相关论文
共 50 条
  • [1] Flexible and transparent supercapacitors using electrospun PEDOT:PSS electrodes
    Cardenas-Martinez, J.
    Espana-Sanchez, Beatriz L.
    Esparza, Rodrigo
    Avila-Nino, Jose A.
    SYNTHETIC METALS, 2020, 267
  • [2] Avoiding Resistance Limitations in High-Performance Transparent Supercapacitor Electrodes Based on Large-Area, High-Conductivity PEDOT:PSS Films
    Higgins, Thomas M.
    Coleman, Jonathan N.
    ACS APPLIED MATERIALS & INTERFACES, 2015, 7 (30) : 16495 - 16506
  • [3] High-performance free-standing PEDOT: PSS electrodes for flexible and transparent all-solid-state supercapacitors
    Cheng, Tao
    Zhang, Yi-Zhou
    Zhang, Jian-Dong
    Lai, Wen-Yong
    Huang, Wei
    JOURNAL OF MATERIALS CHEMISTRY A, 2016, 4 (27) : 10493 - 10499
  • [4] Spray coated high-conductivity PEDOT:PSS transparent electrodes for stretchable and mechanically-robust organic solar cells
    Tait, Jeffrey G.
    Worfolk, Brian J.
    Maloney, Samuel A.
    Hauger, Tate C.
    Elias, Anastasia L.
    Buriak, Jillian M.
    Harris, Kenneth D.
    SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2013, 110 : 98 - 106
  • [5] Stepwise Aggregation Control of PEDOT:PSS Enabled High-Conductivity, High-Resolution Printing of Polymer Electrodes for Transparent Organic Phototransistors
    Xiao, Xixi
    Shen, Xianfeng
    Tie, Yuan
    Zhao, Yaru
    Yang, Ruhe
    Li, Yiming
    Li, Weizhen
    Tang, Liqun
    Li, Rongjin
    Wang, Yi-Xuan
    Hu, Wenping
    ACS APPLIED MATERIALS & INTERFACES, 2024, 16 (22) : 29217 - 29225
  • [6] Hybrid PEDOT:PSS to obtain high-performance Ag NW-based flexible transparent electrodes for transparent heaters
    Xiaopeng Li
    Shihui Yu
    Le Zhao
    Muying Wu
    Helei Dong
    Journal of Materials Science: Materials in Electronics, 2020, 31 : 8106 - 8115
  • [7] Hybrid PEDOT:PSS to obtain high-performance Ag NW-based flexible transparent electrodes for transparent heaters
    Li, Xiaopeng
    Yu, Shihui
    Zhao, Le
    Wu, Muying
    Dong, Helei
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2020, 31 (10) : 8106 - 8115
  • [8] Photolithographic High-Conductivity Transparent Conformal rGO/PEDOT:PSS Electrodes for Flexible Skin-Like All Solution-Processed Organic Transistors
    Wang, Xue
    Zhao, Pengfei
    Tong, Yanhong
    Guo, Shanlei
    Zhao, Guodong
    Zhang, Mingxin
    Yu, Hongyan
    Zhao, Xiaoli
    Tang, Qingxin
    Liu, Yichun
    ADVANCED MATERIALS TECHNOLOGIES, 2022, 7 (12)
  • [9] Inkjet Printable ZnO/PEDOT:PSS Heterojunction for Thin Flexible Semi-Transparent Optoelectronic Sensors
    Frau, Eleonora
    Zhang, Yipeng
    Viau, Lydie
    Jurin, Florian
    Buron, Cedric
    Filiatre, Claudine
    Schintke, Silvia
    2020 22ND INTERNATIONAL CONFERENCE ON TRANSPARENT OPTICAL NETWORKS (ICTON 2020), 2020,
  • [10] Highly Conductive and Transparent PEDOT:PSS Films with a Fluorosurfactant for Stretchable and Flexible Transparent Electrodes
    Vosgueritchian, Michael
    Lipomi, Darren J.
    Bao, Zhenan
    ADVANCED FUNCTIONAL MATERIALS, 2012, 22 (02) : 421 - 428