Selective Hydrogenation of Cinnamaldehyde on Pt and Pt-Fe Catalysts Supported on Zeolite P

被引：20
|
作者：
Neri, G. [1 ,2 ]
Arrigo, I. [2 ]
Corigliano, F. [2 ]
De Luca, L. [3 ]
Donato, A. [3 ]
机构：
[1] Univ Messina Contrada Dio, Dipartimento Chim Ind & Ingn Mat, I-98166 Messina, Italy
[2] Univ Messina, Dept Ind Chem & Mat Engn, I-98166 Messina, Italy
[3] Univ Reggio Calabria, Dept Mech & Mat, I-89100 Reggio Di Calabria, Italy
来源：
CATALYSIS LETTERS | 2011年 / 141卷 / 11期
关键词：
Cinnamaldehyde; Selective hydrogenation; Pt catalysts; Catalytic support; Zeolite P; CINNAMYL ALCOHOL; BETA-ZEOLITE; CAMPHOLENIC ALDEHYDE; CARBON NANOTUBES; PUMICE WASTE; PLATINUM; CO; CROTONALDEHYDE; RUTHENIUM; PROMOTION;
D O I：
10.1007/s10562-011-0688-x
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Pt- and Pt-Fe based catalysts on zeolite P (ZP) support have been prepared and widely characterized by surface area and porosity, XRD, SEM, TEM, TPR, in order to investigate their morphological and microstructural properties. The catalysts have been tested in the selective liquid-phase hydrogenation of cinnamaldehyde. Kinetic tests have shown the beneficial effect of Fe promoter on the catalysts behaviour towards the selective formation of cinnamyl alcohol (85% selectivity to 90% conversion). The ZP supported catalysts have been compared with a catalyst supported on P-zeolitized Fe containing pumice (Z-PM), confirming the role of Fe Lewis acid site in promoting the reactivity of zeolite P-based materials.
引用
收藏
页码：1590 / 1597
页数：8
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