On the viscosity of magnetic fluid with low and moderate solid fraction

被引：27
|
作者：
Ren, Zhiqiang [1 ,2 ]
Han, Yanping [1 ,2 ]
Hong, Ruoyu [1 ,2 ,3 ]
Ding, Hanmin [4 ]
Li, Hongzhong [3 ]
机构：
[1] Soochow Univ, Dept Chem Engn, SIP, Suzhou 215123, Peoples R China
[2] Soochow Univ, Key Lab Organ Synth Jiangsu Prov, SIP, Suzhou 215123, Peoples R China
[3] Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase React, Beijing 100080, Peoples R China
[4] IBM Corp, Rochester, MN 55901 USA
来源：
PARTICUOLOGY | 2008年 / 6卷 / 03期
基金：
中国国家自然科学基金;
关键词：
rheology; capillary rheometer; magnetic fluid; viscosity; Peclet number;
D O I：
10.1016/j.partic.2008.01.004
中图分类号：
TQ [化学工业];
学科分类号：
0817 ;
摘要：
The design of a pressurized capillary rheometer operating at prescribed temperature is described to measure the viscosity of magnetic fluids (MFs) containing Fe3O4 magnetic nanoparticles (MNPs). The equipment constant of the rheometer was obtained using liquids with predetermined viscosities. Experimentally measured viscosities were used to evaluate different equations for suspension viscosities. Deviation of measured suspension viscosities from the Einstein equation was found to be basically due to the influence of spatial distribution and aggregation of Fe3O4 MNPs. By taking account of the coating layer on MNPs and the aggregation of MNPs in MFs, a modified Einstein equation was proposed to fit the experimental data. Moreover, the influence of external magnetic field on viscosity was also taken into account. Viscosities thus predicted are in good agreement with experimental data. Temperature effect on suspension viscosity was shown experimentally to be due to the shear-thinning behavior of the MFs. (c) 2008 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码：191 / 198
页数：8
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