Separating the direct and cascaded contributions to two-dimensional Raman signals using phase-sensitive detection

被引:0
|
作者
Golonzka, O [1 ]
Demirdöven, N [1 ]
Tokmakoff, A [1 ]
机构
[1] MIT, Dept Chem, Cambridge, MA 02139 USA
来源
ULTRAFAST PHENOMENA XII | 2001年 / 66卷
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中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We demonstrate a method of phase-sensitive detection for separating the direct and the cascaded contributions to fifth-order 2-D Raman spectroscopy. The phase of an intrinsic local oscillator is cycled to distinguish the two components that are radiated in quadrature to each other.
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页码:516 / 518
页数:3
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