Quartz crystal microbalance-based method to study adsorption of endocrine disruptor compounds on zeolite

被引:4
|
作者
Li, Wei-Ming [1 ]
Tang, Yu-Jiao [1 ]
Chen, Lin [2 ]
Chen, You-Peng [1 ]
Yan, Peng [1 ]
机构
[1] Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
[2] Army Med Univ, Dept Otorhinolaryngol, Hosp 1, Southwest Hosp, Chongqing, Peoples R China
基金
中国国家自然科学基金;
关键词
Quartz crystal microbalance; environmental endocrine disruptors; zeolite; adsorption; drinking water; 17-ALPHA-ETHINYL ESTRADIOL; AQUEOUS-SOLUTIONS; CARBON NANOTUBES; IONIC-STRENGTH; BISPHENOL-A; REMOVAL; PHARMACEUTICALS; WATER; ACID; 17-BETA-ESTRADIOL;
D O I
10.1080/09593330.2020.1720308
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Endocrine disrupting chemicals (EDCs) can be present as trace-level organic pollutants in aquatic environments and are difficult to measure and remove. In this study, a method was developed using a modified quartz crystal microbalance (QCM) to investigate the adsorption of EDCs by zeolite filter. Bisphenol A (BPA), oestrone (E1), oestradiol (E2), and sulfamethoxazole (SMZ) were selected as four representative endocrine disruptors in a water environment and their adsorption on zeolite was measured by QCM in real-time. The adsorption results were well described by a pseudo-first-order kinetic model and by a Sips isotherms model. The adsorption of the four adsorbents is related to their molecular structure, molecular polarity, and chargeability. The removal rate of EDCs by zeolite for different initial concentrations appeared to plateau, with the removal rates of the four selected EDCs all above 80% except for the maximum initial concentration. Changes of pH and ionic strength had no effect on the adsorption capacity of the four EDCs, with a removal rate of about 90%. However, the response time at pH 5.50 was about 300 s faster than that at pH 8.50 and the addition of electrolyte shortened the mass response time of several organic compounds on QCM.
引用
收藏
页码:3025 / 3035
页数:11
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