Heterospin Junctions in Zigzag-Edged Graphene Nanoribbons

We propose a graphene nanoribbon-based heterojunction, where a defect-free interface separates two zigzag graphene nanoribbons prepared in opposite antiferromagnetic spin configurations. This heterospin junction is found to allow the redirecting of low-energy electrons from one edge to the other. The basic scattering mechanisms and their relation to the system's geometry are investigated through a combination of Landauer-Green's function and the S-matrix and eigen-channel methods within a tight-binding + Hubbard model validated with density functional theory. The findings demonstrate the possibility of using zigzag-edged graphene nanoribbons (zGNRs) in complex networks where current can be transmitted across the entire system, instead of following the shortest paths along connected edges belonging to the same sub-lattice.