Surface Plasmon Enhanced Energy Transfer between Donor and Acceptor CdTe Nanocrystal Quantum Dot Monolayers

被引:159
|
作者
Lunz, Manuela [1 ]
Gerard, Valerie A. [2 ]
Gun'ko, Yurii K. [2 ]
Lesnyak, Vladimir [3 ]
Gaponik, Nikolai [3 ]
Susha, Andrei S. [4 ,5 ]
Rogach, Andrey L. [4 ,5 ]
Bradley, A. Louise [1 ]
机构
[1] Trinity Coll Dublin, Semicond Photon Grp, Sch Phys, Dublin 2, Ireland
[2] Trinity Coll Dublin, Sch Chem, Dublin 2, Ireland
[3] Tech Univ Dresden, D-01062 Dresden, Germany
[4] City Univ Hong Kong, Dept Phys & Mat Sci, Hong Kong, Hong Kong, Peoples R China
[5] City Univ Hong Kong, CFP, Hong Kong, Hong Kong, Peoples R China
基金
爱尔兰科学基金会;
关键词
Quantum dots; nanocrystals; colloidal metal nanoparticles; localized surface plasmons; Forster resonant energy transfer; FLUORESCENCE; CDSE; FRET; LUMINESCENCE; MOLECULES;
D O I
10.1021/nl201714y
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Surface plasmon enhanced Forster resonant energy transfer (FRET) between CdTe nanocrystal quantum dots (QDs) has been observed in a multilayer acceptor QD-gold nanoparticle-donor QD sandwich structure. Compared to a donor-acceptor QD bilayer structure without gold particles, the the FRET rate is enhanced by a factor of 80 and the Forster radius increases by 103%. Furthermore, a strong impact of the donor QD properties on the surface plasmon mediated FRET is reported.
引用
收藏
页码:3341 / 3345
页数:5
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