Aftertreatment Protocols for Catalyst Characterization and Performance Evaluation: Low-Temperature Oxidation, Storage, Three-Way, and NH3-SCR Catalyst Test Protocols

被引:53
|
作者
Rappe, Kenneth G. [1 ]
DiMaggio, Craig [2 ]
Pihl, Josh A. [3 ]
Theis, Joseph R. [4 ]
Oh, Se H. [5 ]
Fisher, Galen B. [6 ]
Parks, Jim [3 ]
Easterling, Vencon G. [2 ]
Yang, Ming [5 ]
Stewart, Mark L. [1 ]
Howden, Kenneth C. [7 ]
机构
[1] Pacific Northwest Natl Lab, Richland, WA 99354 USA
[2] Fiat Chrysler Automobile US FCA USA LLC, 800 Chrysler Dr, Auburn Hills, MI 48326 USA
[3] Oak Ridge Natl Lab, Knoxville, TN 37932 USA
[4] Ford Motor Co, Chem Engn Dept, 2101 Village Rd, Dearborn, MI 48124 USA
[5] Gen Motors Global R&D, 30470 Harley Earl Blvd, Warren, MI 48092 USA
[6] Univ Michigan, Dept Chem Engn, Ann Arbor, MI 48109 USA
[7] US DOE, Energy Efficiency& Renewable Energy, Washington, DC 20585 USA
关键词
Emission control; Three-way catalyst; Oxidation; Selective catalytic reduction; Passive NOx adsorber; Hydrocarbon trap; MULTI-CYLINDER ENGINE; HIGH FUEL EFFICIENCY; NOX; GASOLINE;
D O I
10.1007/s40825-019-00120-7
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A set of standardized and realistic aftertreatment catalyst test protocols have been developed by the Advanced Combustion and Emission Control Technical Team in support of the U.S. DRIVE Partnership. The protocols are intended to accelerate the pace of aftertreatment catalyst innovation by enabling the accurate evaluation and comparison of aftertreatment catalyst performance data from various testing and research facilities to maximize the impact of discovery-phase research occurring across the nation. The protocols address a need identified by the Partnership's industry partners for consistent and accurate metrics for aftertreatment catalyst evaluation and comparison. The protocols consist of a set of standardized requirements and test procedures that sufficiently capture the performance capability of a catalyst technology in a manner that is adaptable in various laboratories. The protocols provide a detailed description of the necessary reactor system, the steps for achieving a desired aged state of the catalyst, all necessary sample pretreatments to be performed prior to testing, and realistic test conditions for evaluating performance. This article details four low-temperature catalyst test protocols applicable to (1) oxidation catalysts, (2) passive storage (and release) catalysts, (3) three-way catalysts, and (4) NH3-SCR catalysts. The catalyst test protocol descriptions are presented in five (5) sections: protocol general guidelines and the four individual catalyst test protocol descriptions. The general guidelines plus the individual protocol description forms the complete low-temperature catalyst test protocol for the application.
引用
收藏
页码:183 / 214
页数:32
相关论文
共 50 条
  • [1] Aftertreatment Protocols for Catalyst Characterization and Performance Evaluation: Low-Temperature Oxidation, Storage, Three-Way, and NH3-SCR Catalyst Test Protocols
    Kenneth G. Rappé
    Craig DiMaggio
    Josh A. Pihl
    Joseph R. Theis
    Se H. Oh
    Galen B. Fisher
    Jim Parks
    Vencon G. Easterling
    Ming Yang
    Mark L. Stewart
    Kenneth C. Howden
    Emission Control Science and Technology, 2019, 5 : 183 - 214
  • [2] A superior MnNiAlOx catalyst for low-temperature NH3-SCR: Performance enhancement and denitration mechanism
    Luan, Xinru
    Yang, Zhuo
    Zhai, Yujia
    Wang, Mengmeng
    Liu, Wei
    Wang, Liguo
    Wang, Zhongpeng
    FUEL, 2024, 376
  • [3] Low-temperature NH3-SCR performance of a novel Chlorella@Mn composite denitrification catalyst
    Liu, Hengheng
    Gao, Fengyu
    Ko, Songjin
    Luo, Ning
    Tang, Xiaolong
    Duan, Erhong
    Yi, Honghong
    Zhou, Yuansong
    JOURNAL OF ENVIRONMENTAL SCIENCES, 2024, 137 : 271 - 286
  • [4] Enhanced low-temperature NH3-SCR performance of CeTiOx catalyst via surface Mo modification
    Li, Lulu
    Li, Peixiao
    Tan, Wei
    Ma, Kaili
    Zou, Weixin
    Tang, Changjin
    Dong, Lin
    CHINESE JOURNAL OF CATALYSIS, 2020, 41 (02) : 364 - 373
  • [5] Low-temperature Denitration Mechanism of NH3-SCR over Fe/AC Catalyst
    Yang, Zhengyu
    Huang, Bangfu
    Zhang, Guifang
    Dai, Meng
    Wen, Zhenjing
    Li, Wanjun
    JOURNAL OF WUHAN UNIVERSITY OF TECHNOLOGY-MATERIALS SCIENCE EDITION, 2023, 38 (03): : 475 - 484
  • [6] Low-temperature Denitration Mechanism of NH3-SCR over Fe/AC Catalyst
    杨征宇
    黄帮福
    ZHANG Guifang
    DAI Meng
    WEN Zhenjing
    LI Wanjun
    JournalofWuhanUniversityofTechnology(MaterialsScience), 2023, 38 (03) : 475 - 484
  • [7] Low-temperature Denitration Mechanism of NH3-SCR over Fe/AC Catalyst
    Zhengyu Yang
    Bangfu Huang
    Guifang Zhang
    Meng Dai
    Zhenjing Wen
    Wanjun Li
    Journal of Wuhan University of Technology-Mater. Sci. Ed., 2023, 38 : 475 - 484
  • [8] Improvement of Low-Temperature Activity of FeBeta Monolith Catalyst in NH3-SCR of NOx
    Alina I. Mytareva
    Dmitriy A. Bokarev
    Dmitriy S. Krivoruchenko
    Galina N. Baeva
    Alexey Yu. Belyankin
    Alexander Yu. Stakheev
    Topics in Catalysis, 2019, 62 : 86 - 92
  • [9] Improvement of Low-Temperature Activity of FeBeta Monolith Catalyst in NH3-SCR of NOx
    Mytareva, Alina I.
    Bokarev, Dmitriy A.
    Krivoruchenko, Dmitriy S.
    Baeva, Galina N.
    Belyankin, Alexey Yu.
    Stakheev, Alexander Yu.
    TOPICS IN CATALYSIS, 2019, 62 (1-4) : 86 - 92
  • [10] Novel MnWOx catalyst with remarkable performance for low temperature NH3-SCR of NOx
    Liu, Fudong
    Shan, Wenpo
    Lian, Zhihua
    Xie, Lijuan
    Yang, Weiwei
    He, Hong
    CATALYSIS SCIENCE & TECHNOLOGY, 2013, 3 (10) : 2699 - 2707