Mode-coupling theory for tagged-particle motion of active Brownian particles

被引:14
|
作者
Reichert, Julian [1 ]
Mandal, Suvendu [2 ,3 ]
Voigtmann, Thomas [1 ,2 ]
机构
[1] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Mat Phys Weltraum, D-51170 Cologne, Germany
[2] Heinrich Heine Univ Dusseldorf, Dept Phys, Univ Str 1, D-40225 Dusseldorf, Germany
[3] Tech Univ Darmstadt, Inst Phys Kondensierten Materie, D-64289 Darmstadt, Germany
关键词
NONEQUILIBRIUM GLASSY DYNAMICS; LONG-WAVELENGTH FLUCTUATIONS; ASYMPTOTIC LAWS; TRANSITION; CELL; DIFFUSION;
D O I
10.1103/PhysRevE.104.044608
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We derive a mode-coupling theory (MCT) to describe the dynamics of a tracer particle that is embedded in a dense system of active Brownian particles (ABPs) in two spatial dimensions. The ABP undergo translational and rotational Brownian motion and are equipped with a fixed self-propulsion speed along their orientational vector that describes their active motility. The resulting equations of motion for the tagged-particle densitycorrelation functions describe the various cases of tracer dynamics close to the glass transition: that of a single active particle in a glass-forming passive host suspensions, that of a passive colloidal particle in a suspension of ABP, and that of active tracers in a bath of active particles. Numerical results are presented for these cases assuming hard-sphere interactions among the particles. The qualitative and quantitative accuracy of the theory is tested against event-driven Brownian dynamics (ED-BD) simulations of active and passive hard disks. Simulation and theory are found in quantitative agreement, provided one adjusts the overall density (as known from the passive description of glassy dynamics), and allows for a rescaling of self-propulsion velocities in the active host system. These adjustments account for the fact that ABP-MCT generally overestimates the tendency for kinetic arrest. We confirm in the simulations a peculiar feature of the transient and stationary dynamical density-correlation functions regarding their lack of symmetry under time reversal, demonstrating the nonequilibrium nature of the system and how it manifests itself in the theory.
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页数:17
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