Energy flows in graphene: hot carrier dynamics and cooling

被引:64
|
作者
Song, Justin C. W. [1 ,2 ]
Levitov, Leonid S. [1 ]
机构
[1] MIT, Dept Phys, Cambridge, MA 02139 USA
[2] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
关键词
light-matter interaction; electron-lattice cooling; supercollisions; LOSS RATES; PHOTOCURRENT; RELAXATION; TRANSPORT; SUPERCOLLISIONS; MULTIPLICATION; PHOTORESPONSE; CONDUCTIVITY; ABSORPTION; SCATTERING;
D O I
10.1088/0953-8984/27/16/164201
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Long lifetimes of hot carriers can lead to qualitatively new types of responses in materials. The magnitude and time scales for these responses reflect the mechanisms governing energy flows. We examine the microscopics of two processes which are key for energy transport, focusing on the unusual behavior arising due to graphene's unique combination of material properties. One is hot carrier generation in its photoexcitation dynamics, where hot carriers multiply through an Auger type carrier-carrier scattering cascade. The hot-carrier generation manifests itself through elevated electronic temperatures which can be accessed in a variety of ways, in particular optical conductivity measurements. Another process of high interest is electron-lattice cooling. We survey different cooling pathways and discuss the cooling bottleneck arising for the momentum-conserving electron-phonon scattering pathway. We show how this bottleneck can be relieved by higher-order collisions-supercollisions-and examine the variety of supercollision processes that can occur in graphene.
引用
收藏
页数:15
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