Translocation events in a single-walled carbon nanotube

被引:15
|
作者
He, Jin [1 ]
Liu, Hao [2 ]
Pang, Pei [3 ]
Cao, Di [3 ]
Lindsay, Stuart [1 ,2 ,3 ]
机构
[1] Arizona State Univ, Biodesign Inst, Tempe, AZ 85287 USA
[2] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA
[3] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA
关键词
MASS-TRANSPORT; STRANDED-DNA; WATER; MOLECULES; CHANNEL;
D O I
10.1088/0953-8984/22/45/454112
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Translocation of DNA oligomers through a single-walled carbon nanotube was demonstrated recently. Translocation events are accompanied by giant current pulses, the origin of which remains obscure. Here, we show that the introduction of a nucleotide, guanosine triphosphate, alone into the input reservoir of a carbon nanotube nanofluidic device also gives giant current pulses. Taken together with data on oligomer translocation, these new results suggest that the pulse width has a nonlinear, power-law dependence on the number of nucleotides in a DNA molecule. We have also measured the time for the onset of DNA translocation pulses after bias reversal, finding that the time for the onset of translocation is directly proportional to the period of the bias reversal.
引用
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页数:6
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