Three separate estimates of ozone trends since 1970 are obtained from ozonesonde analyses in the Northern Hemisphere, at up to 11 point locations. Our analysis shows that there has been an increase in the annually averaged tropopause height of between 330-520 m at all stations, accompanied by an overall upward movement of the ozone profile. This movement of the ozone profile has led to an extra 2-15% decade(-1) ozone depletion between roughly 8 and 22 km. We argue that as the part of the ozone trend associated with "dynamical" movement of the ozone profile is not a direct result of anthropogenic chemical ozone depletion, it ought not to be included in anthropogenic radiative forcing calculations. This leads to a stratospheric ozone radiative forcing which is roughly 50% of the original estimate. Combining stratospheric and tropospheric ozone changes to calculate the total ozone radiative forcing in the Northern Hemisphere for the 1970-1997 period gives a radiative forcing of -0.09 W m(-2), excluding the effects of dynamical movement of the ozone profile, which were calculated to have led to a further "ozone feedback" of -0.1 W m(-2). These results suggest estimating ozone radiative forcing from observational ozone trend data, without accounting for the movement of the ozone profile could be fundamentally flawed, due to the unquantified feedbacks in the climate system, making it difficult to separate out the part of the ozone trend associated directly with the anthropogenic forcing.
机构:
Columbia Univ, Dept Appl Phys & Appl Math, New York, NY USAColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Son, Seok-Woo
Polvani, Lorenzo M.
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Columbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Columbia Univ, Dept Earth & Environm Sci, New York, NY USAColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Polvani, Lorenzo M.
Waugh, Darryn W.
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Johns Hopkins Univ, Dept Earth & Planetary Sci, Baltimore, MD 21218 USAColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Waugh, Darryn W.
Birner, Thomas
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Univ Toronto, Dept Phys, Toronto, ON, CanadaColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Birner, Thomas
Akiyoshi, Hideharu
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Natl Inst Environm Studies, Tsukuba, Ibaraki, JapanColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Akiyoshi, Hideharu
Garcia, Rolando R.
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Natl Ctr Atmospher Res, Boulder, CO 80307 USAColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Garcia, Rolando R.
Gettelman, Andrew
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Natl Ctr Atmospher Res, Boulder, CO 80307 USAColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Gettelman, Andrew
Plummer, David A.
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Environm Canada, Toronto, ON, CanadaColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
Plummer, David A.
Rozanov, Eugene
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机构:
ETH, Inst Atmospher & Climate Sci, Zurich, Switzerland
World Radiat Ctr, Phys Meteorol Observ, Davos, SwitzerlandColumbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
机构:
Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USALawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Santer, BD
Wehner, MF
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Wehner, MF
Wigley, TML
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Wigley, TML
Sausen, R
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Sausen, R
Meehl, GA
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Meehl, GA
Taylor, KE
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Taylor, KE
Ammann, C
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Ammann, C
Arblaster, J
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Arblaster, J
Washington, WM
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Washington, WM
Boyle, JS
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Boyle, JS
Brüggemann, W
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
机构:
Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USALawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Santer, BD
Wehner, MF
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h-index: 0
机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Wehner, MF
Wigley, TML
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h-index: 0
机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Wigley, TML
Sausen, R
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h-index: 0
机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Sausen, R
Meehl, GA
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Meehl, GA
Taylor, KE
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Taylor, KE
Ammann, C
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Ammann, C
Arblaster, J
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Arblaster, J
Washington, WM
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Washington, WM
Boyle, JS
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA
Boyle, JS
Brüggemann, W
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机构:Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA