Crystal-field excitations in multiferroic TbMnO3 by Mn L3 and O K resonant inelastic X-ray scattering

被引：0
|
作者：
Feng, Jiatai [1 ]
Juhin, Amelie [2 ]
Delaunay, Renaud [1 ,3 ]
Jarrier, Romain [1 ,3 ]
Jaouen, Nicolas [3 ]
Nicolaou, Alessandro [3 ]
Sinclair, Ryan [4 ]
Zhou, Haidong [4 ]
Mariot, Jean-Michel [1 ,3 ]
Chiuzbaian, Sorin G. [1 ,3 ]
机构：
[1] UPMC Univ Paris 06, Sorbonne Univ, Lab Chim Phys Mat & Rayonnement UMR 7614, CNRS, 4 Pl Jussieu, F-75252 Paris 05, France
[2] UPMC Univ Paris 06, Sorbonne Univ, Inst Mineral Phys Mat & Cosmochim UMR 7590, CNRS,IRD,MNHN, 4 Pl Jussieu, F-75252 Paris 05, France
[3] Synchrotron SOLEIL, BP 48, F-91192 Gif Sur Yvette, France
[4] Univ Tennessee, Dept Phys & Astron, Expt Condensed Matter Phys, 407A Nielsen Phys Bldg, Knoxville, TN 37996 USA
来源：
JOURNAL OF APPLIED PHYSICS | 2017年 / 122卷 / 19期
关键词：
OXYGEN; MANGANITES; EMISSION; STATE;
D O I：
10.1063/1.4990683
中图分类号：
O59 [应用物理学];
学科分类号：
摘要：
d-d excitations in multiferroic TbMnO3 have been investigated by X-ray absorption spectroscopy and resonant inelastic X-ray scattering at the Mn L-3,L-2 and O K edges. Confrontation between experimental data and multiplet crystal-field calculations performed for Mn3+ ions in D-4h symmetry has enabled us to identify the origin of the observed excitations and has provided reliable manganese crystal-field parameters that enter the description of the antisymmetric exchange interaction responsible for the multiferroicity in this compound. Published by AIP Publishing.
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页数：6
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